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Effect of hydrophobized PET TeMs membrane pore-size on saline water treatment by direct contact membrane distillation.

ABSTRACT: This paper describes the desalination process by membrane distillation (MD) using track-etched membranes (TeMs). Hydrophobic track-etched membranes based on poly(ethylene terephthalate) (PET TeMs) with pore diameters from 700 to 1300 nm were prepared by UV-initiated graft polymerization of lauryl methacrylate (LMA) inside the nanochannels. Modified PET TeMs were investigated by Fourier transform infrared (FTIR) spectroscopy, atomic force microscopy (AFM), scanning electron microscopy (SEM), thermogravimetric analysis (TGA) and contact wetting angle (CA) measurements. Hydrophobic PET TeMs were tested for treating saline solutions of different concentrations by the direct contact membrane distillation (DCMD) method. The influence of membrane pore diameter and salt solution concentration on the water flux and rejection degree were investigated. Membranes with CA 94 ± 4° were tested in the direct contact membrane distillation (DCMD) of 7.5-30 g L^-1 saline solution. Hydrophobic membranes with large pore sizes showed water fluxes in the range of 1.88 to 11.70 kg m^-2 h^-1 with salt rejection values of up to 91.4%.

SUBMITTER: Yeszhanov AB

PROVIDER: S-EPMC10823361 | biostudies-literature | 2024 Jan

REPOSITORIES: biostudies-literature

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Effect of hydrophobized PET TeMs membrane pore-size on saline water treatment by direct contact membrane distillation.

Yeszhanov Arman B AB Korolkov Ilya V IV Güven Olgun O Melnikova Galina B GB Dosmagambetova Saule S SS Borissenko Alexander N AN Nurkassimov A K AK Kassymzhanov Murat T MT Zdorovets Maxim V MV

RSC advances 20240129 6

This paper describes the desalination process by membrane distillation (MD) using track-etched membranes (TeMs). Hydrophobic track-etched membranes based on poly(ethylene terephthalate) (PET TeMs) with pore diameters from 700 to 1300 nm were prepared by UV-initiated graft polymerization of lauryl methacrylate (LMA) inside the nanochannels. Modified PET TeMs were investigated by Fourier transform infrared (FTIR) spectroscopy, atomic force microscopy (AFM), scanning electron microscopy (SEM), ther ...[more]

PMID: 38288145

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Project description:Direct Contact Membrane Distillation (DCMD) is a promising and feasible technology for water desalination. Most of the models used to simulate DCMD are one-dimensional and/or use a linear function of vapour pressure which relies on experimentally determined parameters. In this study, the model of DCMD using Nusselt correlations was improved by coupling the continuity, momentum, and energy equations to better capture the downstream alteration of flow field properties. A logarithmic function of vapour pressure, which is independent from experiments, was used. This allowed us to analyse DCMD with different membrane properties. The results of our developed model were in good agreement with the DCMD experimental results, with less than 7% deviation. System performance metrics, including water flux, temperature, and concentration polarisation coefficient and thermal efficiency, were analysed by varying inlet feed and permeate temperature, inlet velocity, inlet feed concentration, channel length. In addition, twenty-two commercial membranes were analysed to obtain a real vision on the influence of membrane characteristics on system performance metrics. The results showed that the feed temperature had the most significant effect on water flux and thermal efficiency. The increased feed temperature enhanced the water flux and thermal efficiency; however, it caused more concentration and temperature polarisation. On the other hand, the increased inlet velocity was found to provide increased water flux and reduced temperature and concertation polarisation as well. It was also found that the membrane properties, especially thickness and porosity, can affect the DCMD performance significantly. A two-fold increase of feed temperature increased the water flux and thermal efficiency, 10-fold and 27%, respectively; however, it caused an increase in temperature and concertation polarisation, at 48% and 34%, respectively. By increasing Reynolds number from 80 to 1600, the water flux, CPC, and TPC enhanced by 2.3-fold, 2%, and 21%, respectively. The increased feed concentration from 0 to 250 [g/L] caused a 26% reduction in water flux. To capture the downstream alteration of flow properties, it was shown that the ratio of inlet value to outlet value of system performance metrics decreased significantly throughout the module. Therefore, improvement over the conventional model is undeniable, as the new model can assist in achieving optimal operation conditions.

Dataset Information

Effect of hydrophobized PET TeMs membrane pore-size on saline water treatment by direct contact membrane distillation.

Publications

Effect of hydrophobized PET TeMs membrane pore-size on saline water treatment by direct contact membrane distillation.

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