Unknown

Dataset Information

0

Tailoring of magnetism & electron transport of manganate thin films by controlling the Mn-O-Mn bond angles via strain engineering.

ABSTRACT: Strain engineering beyond substrate limitation of colossal magnetoresistant thin (La0.6Pr0.4)0.7Ca0.3MnO3 (LPCMO) films on LaAlO3-buffered SrTiO3 (LAO/STO) substrates has been demonstrated using metalorganic aerosol deposition technique. By growing partially relaxed 7-27 nm thick heteroepitaxial LAO buffer layers on STO a perfect lattice matching to the LPCMO has been achieved. As a result, strain-free heteroepitaxial 10-20 nm thick LPCMO/LAO/STO films with bulk-like ferromagnetic metallic ground state were obtained. Without buffer the coherently strained thin LPCMO/STO and LPCMO/LAO films were insulating and weakly magnetic. The reason for the optimized magnetotransport in strain-free LPCMO films was found to be a large octahedral Mn-O-Mn bond angle φOOR ~ 166-168° as compared to the significantly smaller one of φOOR ~ 152-156° determined for the tensile (LPCMO/STO) and compressively (LPCMO/LAO) strained films.

SUBMITTER: Henning P 

PROVIDER: S-EPMC10853165 | biostudies-literature | 2024 Feb

REPOSITORIES: biostudies-literature

Json Xml
altmetric image

Publications

Tailoring of magnetism & electron transport of manganate thin films by controlling the Mn-O-Mn bond angles via strain engineering.

Henning P P   Gruhl R R   Ross U U   Roddatis V V   Bruchmann-Bamberg V V   Stroh K P KP   Seibt M M   Gegenwart P P   Moshnyaga V V  

Scientific reports 20240208 1

Strain engineering beyond substrate limitation of colossal magnetoresistant thin (La<sub>0.6</sub>Pr<sub>0.4</sub>)<sub>0.7</sub>Ca<sub>0.3</sub>MnO<sub>3</sub> (LPCMO) films on LaAlO<sub>3</sub>-buffered SrTiO<sub>3</sub> (LAO/STO) substrates has been demonstrated using metalorganic aerosol deposition technique. By growing partially relaxed 7-27 nm thick heteroepitaxial LAO buffer layers on STO a perfect lattice matching to the LPCMO has been achieved. As a result, strain-free heteroepitaxial 1  ...[more]

Similar Datasets

Unknown Emergent Magnetic Phenomenon with Unconventional Structure in Epitaxial Manganate Thin Films.
| S-EPMC8261492 | biostudies-literature
Unknown Reversible control of magnetism in FeRh thin films.
| S-EPMC7435192 | biostudies-literature
Unknown Carrier dynamics of Mn-induced states in GaN thin films.
| S-EPMC5517569 | biostudies-literature
Unknown Tailoring of Multisource Deposition Conditions towards Required Chemical Composition of Thin Films
| S-EPMC9182166 | biostudies-literature
Unknown Reversible, Electric-Field Induced Magneto-Ionic Control of Magnetism in Mesoporous Cobalt Ferrite Thin Films.
| S-EPMC6658663 | biostudies-literature
Unknown The effect of Mn2Sb2 and Mn2Sb secondary phases on magnetism in (GaMn)Sb thin films.
| S-EPMC7159204 | biostudies-literature
Unknown Quantitative Analysis of Electron Beam Damage in Organic Thin Films.
| S-EPMC5442601 | biostudies-literature
Unknown Tailoring magnetic properties of multicomponent layered structure via current annealing in FePd thin films.
| S-EPMC5709423 | biostudies-literature
Unknown Tailoring the nanoscale morphology of HKUST-1 thin films via codeposition and seeded growth.
| S-EPMC5687001 | biostudies-literature
Unknown Tailoring magnetism in silicon-doped zigzag graphene edges.
| S-EPMC9338279 | biostudies-literature