Project description:Combining bright-field and edge-enhanced imaging affords an effective avenue for extracting complex morphological information from objects, which is particularly beneficial for biological imaging. Multiplexing meta-lenses present promising candidates for achieving this functionality. However, current multiplexing meta-lenses lack spectral modulation, and crosstalk between different wavelengths hampers the imaging quality, especially for biological samples requiring precise wavelength specificity. Here, we experimentally demonstrate the nonlocal Huygens' meta-lens for high-quality-factor spin-multiplexing imaging. Quasi-bound states in the continuum (q-BICs) are excited to provide a high quality factor of 90 and incident-angle dependence. The generalized Kerker condition, driven by Fano-like interactions between q-BIC and in-plane Mie resonances, breaks the radiation symmetry, resulting in a transmission peak with a geometric phase for polarization-converted light, while unconverted light exhibits a transmission dip without a geometric phase. Enhanced polarization conversion efficiency of 65% is achieved, accompanied by a minimal unconverted value, surpassing the theoretical limit of traditional thin nonlocal metasurfaces. Leveraging these effects, the output polarization-converted state exhibits an efficient wavelength-selective focusing phase profile. The unconverted counterpart serves as an effective spatial frequency filter based on incident-angular dispersion, passing high-frequency edge details. Bright-field imaging and edge detection are thus presented under two output spin states. This work provides a versatile framework for nonlocal metasurfaces, boosting biomedical imaging and sensing applications.
Project description:ABSTRACT Momentum-space polarization vortices centered at symmetry-protected bound states in the continuum of a periodic structure, e.g. photonic crystal slab, provide a novel nonlocal approach to generate vortex beams. This approach enjoys a great convenience of no precise alignment requirements, although the generation efficiency of the nonlocal generators requires further optimization before the practical application. In this work, we propose a temporal-coupled-mode-theory-based guideline for high-efficiency nonlocal reflection-type vortex generator design. The conversion efficiency of the vortex beam is found to be limited by the ratio of the radiative loss to the intrinsic absorption in practical systems. To increase this ratio through mode selection and structure design, the photonic crystal slabs are theoretically designed and experimentally characterized, showing a maximum on-resonance conversion efficiency of up to 86%. Combining high efficiency with simple fabrication and no requirement for precise alignment, reflection-type photonic crystal slabs could offer a new and competitive way to generate vortex beams flexibly.
Project description:Trapping electromagnetic waves within the radiation continuum holds significant implications in the field of optical science and technology. Photonic bound states in the continuum (BICs) present a distinctive approach for achieving this functionality, offering potential applications in laser systems, sensing technologies, and other domains. However, the simultaneous achievement of high Q-factors, flat-band dispersions, and wide-angle responses in photonic BICs has not yet been reported, thereby impeding their practical performance due to laser direction deviation or sample disorder. Here, we theoretically demonstrate the construction of moiré BICs in one-dimensional photonic crystal (PhC) slabs, where high-Q resonances in the entire moiré flat band are achieved. Specifically, we numerically validate that the radiation loss of moiré BICs can be eliminated by aligning multiple topological polarization charges with all diffraction channels, enabling the strong suppression of far-field radiation from the entire moiré band. This leads to a slow decay of Q-factors away from moiré BICs in the momentum space. Moreover, it is found that Q-factors of the moiré flat band can still maintain at a high level with structural disorder. In experiments, we fabricate the designed 1D moiré PhC slab and observe both high-Q resonances and a slow decrease of Q-factors for moiré flat-band Bloch modes. Our findings hold promising implications for designing highly efficient optical devices with wide-angle responses and introduce a novel avenue for exploring BICs in moiré superlattices.
Project description:Enhancing light-matter interactions is fundamental to the advancement of nanophotonics and optoelectronics. Yet, light diffraction on dielectric platforms and energy loss on plasmonic metallic systems present an undesirable trade-off between coherent energy exchange and incoherent energy damping. Through judicious structural design, both light confinement and energy loss issues could be potentially and simultaneously addressed by creating bound states in the continuum (BICs) where light is ideally decoupled from the radiative continuum. Herein, the authors present a general framework based on the two-coupled resonances to first conceptualize and then numerically demonstrate a type of quasi-BICs that can be achieved through the interference between two bare resonance modes and is characterized by the considerably narrowed spectral line shape even on lossy metallic nanostructures. The ubiquity of the proposed framework further allows the paradigm to be extended for the realization of plexcitonic quasi-BICs on the same metallic systems. Owing to the topological nature, both plasmonic and plexcitonic quasi-BICs display strong mode robustness against parameters variation, thereby providing an attractive platform to unlock the potential of the coupled plasmon-exciton systems for manipulation of the photophysical properties of condensed phases.
Project description:Quantum mechanics predicts that certain stationary potentials can sustain bound states with an energy buried in the continuous spectrum of scattered states, the so-called bound states in the continuum (BIC). Originally regarded as mathematical curiosities, BIC have found an increasing interest in recent years, particularly in quantum and classical transport of matter and optical waves in mesoscopic and photonic systems where the underlying potential can be judiciously tailored. Most of our knowledge of BIC is so far restricted to static potentials. Here we introduce a new kind of BIC, referred to as Floquet BIC, which corresponds to a normalizable Floquet state of a time-periodic Hamiltonian with a quasienergy embedded into the spectrum of Floquet scattered states. We discuss the appearance of Floquet BIC states in a tight-binding lattice model driven by an ac field in the proximity of the dynamic localization regime.
Project description:Chipscale micro- and nano-optomechanical systems, hinging on the intangible radiation-pressure force, have shown their unique strength in sensing, signal transduction, and exploration of quantum physics with mechanical resonators. Optomechanical crystals, as one of the leading device platforms, enable simultaneous molding of the band structure of optical photons and microwave phonons with strong optomechanical coupling. Here, we demonstrate a new breed of optomechanical crystals in two-dimensional slab-on-substrate structures empowered by mechanical bound states in the continuum (BICs) at 8 GHz. We show symmetry-induced BIC emergence with optomechanical couplings up to g/2π ≈ 2.5 MHz per unit cell, on par with low-dimensional optomechanical crystals. Our work paves the way towards exploration of photon-phonon interaction beyond suspended microcavities, which might lead to new applications of optomechanics from phonon sensing to quantum transduction.
Project description:Photocatalytic platforms based on ultrathin reactive materials facilitate carrier transport and extraction but are typically restricted to a narrow set of materials and spectral operating ranges due to limited absorption and poor energy-tuning possibilities. Metasurfaces, a class of 2D artificial materials based on the electromagnetic design of nanophotonic resonators, allow optical absorption engineering for a wide range of materials. Moreover, tailored resonances in nanostructured materials enable strong absorption enhancement and thus carrier multiplication. Here, we develop an ultrathin catalytic metasurface platform that leverages the combination of loss-engineered substoichiometric titanium oxide (TiO2-x) and the emerging physical concept of optical bound states in the continuum (BICs) to boost photocatalytic activity and provide broad spectral tunability. We demonstrate that our platform reaches the condition of critical light coupling in a TiO2-x BIC metasurface, thus providing a general framework for maximizing light-matter interactions in diverse photocatalytic materials. This approach can avoid the long-standing drawbacks of many naturally occurring semiconductor-based ultrathin films applied in photocatalysis, such as poor spectral tunability and limited absorption manipulation. Our results are broadly applicable to fields beyond photocatalysis, including photovoltaics and photodetectors.
Project description:Non-radiative bound states in the continuum (BICs) allow construction of resonant cavities with confined electromagnetic energy and high-quality (Q) factors. However, the sharp decay of the Q factor in the momentum space limits their usefulness for device applications. Here we demonstrate an approach to achieve sustainable ultrahigh Q factors by engineering Brillouin zone folding-induced BICs (BZF-BICs). All the guided modes are folded into the light cone through periodic perturbation that leads to the emergence of BZF-BICs possessing ultrahigh Q factors throughout the large, tunable momentum space. Unlike conventional BICs, BZF-BICs show perturbation-dependent dramatic enhancement of the Q factor in the entire momentum space and are robust against structural disorders. Our work provides a unique design path for BZF-BIC-based silicon metasurface cavities with extreme robustness against disorder while sustaining ultrahigh Q factors, offering potential applications in terahertz devices, nonlinear optics, quantum computing, and photonic integrated circuits.
Project description:Photonic bound states in the continuum (BICs), embedded in the spectrum of free-space waves1,2 with diverging radiative quality factor, are topologically non-trivial dark modes in open-cavity resonators that have enabled important advances in photonics3,4. However, it is particularly challenging to achieve maximum near-field enhancement, as this requires matching radiative and non-radiative losses. Here we propose the concept of supercritical coupling, drawing inspiration from electromagnetically induced transparency in near-field coupled resonances close to the Friedrich-Wintgen condition2. Supercritical coupling occurs when the near-field coupling between dark and bright modes compensates for the negligible direct far-field coupling with the dark mode. This enables a quasi-BIC field to reach maximum enhancement imposed by non-radiative loss, even when the radiative quality factor is divergent. Our experimental design consists of a photonic-crystal nanoslab covered with upconversion nanoparticles. Near-field coupling is finely tuned at the nanostructure edge, in which a coherent upconversion luminescence enhanced by eight orders of magnitude is observed. The emission shows negligible divergence, narrow width at the microscale and controllable directivity through input focusing and polarization. This approach is relevant to various physical processes, with potential applications for light-source development, energy harvesting and photochemical catalysis.
Project description:While structural colors are ubiquitous in nature, saturated reds are mysteriously absent. This long-standing problem of achieving Schrödinger's red demands sharp transitions from "stopband" to a high-reflectance "passband" with total suppression of higher-order resonances at blue/green wavelengths. Current approaches based on nanoantennas are insufficient to satisfy all conditions simultaneously. Here, we designed Si nanoantennas to support two partially overlapping quasi-bound-states-in-the-continuum modes with a gradient descent algorithm to achieve sharp spectral edges at red wavelengths. Meanwhile, high-order modes at blue/green wavelengths are suppressed via engineering the substrate-induced diffraction channels and the absorption of amorphous Si. This design produces possibly the most saturated and brightest reds with ~80% reflectance, exceeding the red vertex in sRGB and even the cadmium red pigment. Its nature of being sensitive to polarization and illumination angle could be potentially used for information encryption, and this proposed paradigm could be generalized to other Schrödinger's color pixels.