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Splitting CO2 into CO and O2 by a single catalyst.

ABSTRACT: The metal complex [(tpy)(Mebim-py)Ru(II)(S)](2+) (tpy = 2,2' : 6',2''-terpyridine; Mebim-py = 3-methyl-1-pyridylbenzimidazol-2-ylidene; S = solvent) is a robust, reactive electrocatalyst toward both water oxidation to oxygen and carbon dioxide reduction to carbon monoxide. Here we describe its use as a single electrocatalyst for CO(2) splitting, CO(2) ? CO + 1/2 O(2), in a two-compartment electrochemical cell.

SUBMITTER: Chen Z 

PROVIDER: S-EPMC3465442 | biostudies-literature | 2012 Sep

REPOSITORIES: biostudies-literature

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Splitting CO2 into CO and O2 by a single catalyst.

Chen Zuofeng Z   Concepcion Javier J JJ   Brennaman M Kyle MK   Kang Peng P   Norris Michael R MR   Hoertz Paul G PG   Meyer Thomas J TJ  

Proceedings of the National Academy of Sciences of the United States of America 20120608 39

The metal complex [(tpy)(Mebim-py)Ru(II)(S)](2+) (tpy = 2,2' : 6',2''-terpyridine; Mebim-py = 3-methyl-1-pyridylbenzimidazol-2-ylidene; S = solvent) is a robust, reactive electrocatalyst toward both water oxidation to oxygen and carbon dioxide reduction to carbon monoxide. Here we describe its use as a single electrocatalyst for CO(2) splitting, CO(2) → CO + 1/2 O(2), in a two-compartment electrochemical cell. ...[more]

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