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Two-photon-coincidence fluorescence spectra of cavity multipolaritons: novel signatures of multiexciton generation.


ABSTRACT: In a simulation study, we show that correlated two-dimensional frequency-resolved fluorescence spectra of a quantum dot in a microcavity provide a sensitive probe for the distribution of multiexcitons. Polariton couplings lead to a fine structure of Rabi multiplets that allow us to resolve otherwise overlapping features of the different multiexcitons. These may be used to probe multiexciton generation.

SUBMITTER: Roslyak O 

PROVIDER: S-EPMC3721745 | biostudies-literature | 2010 Oct

REPOSITORIES: biostudies-literature

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Two-photon-coincidence fluorescence spectra of cavity multipolaritons: novel signatures of multiexciton generation.

Roslyak Oleksiy O   Gumbs Godfrey G   Mukamel Shaul S  

Nano letters 20101001 10


In a simulation study, we show that correlated two-dimensional frequency-resolved fluorescence spectra of a quantum dot in a microcavity provide a sensitive probe for the distribution of multiexcitons. Polariton couplings lead to a fine structure of Rabi multiplets that allow us to resolve otherwise overlapping features of the different multiexcitons. These may be used to probe multiexciton generation. ...[more]

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