Unknown

Dataset Information

0

Gelling by heating.


ABSTRACT: We exploit the concept of competing interactions to design a binary mixture of patchy particles that forms a reversible gel upon heating. Our molecular dynamics computer simulation of such a system shows that with increasing temperature the relaxation dynamics slows down by more than four orders of magnitude and then speeds up again. The system is thus a fluid both at high and at low temperatures and a solid-like disordered open network structure at intermediate temperature. We further discuss the feasibility of realizing a real material with this reversible behavior.

SUBMITTER: Roldan-Vargas S 

PROVIDER: S-EPMC3744795 | biostudies-literature | 2013

REPOSITORIES: biostudies-literature

altmetric image

Publications


We exploit the concept of competing interactions to design a binary mixture of patchy particles that forms a reversible gel upon heating. Our molecular dynamics computer simulation of such a system shows that with increasing temperature the relaxation dynamics slows down by more than four orders of magnitude and then speeds up again. The system is thus a fluid both at high and at low temperatures and a solid-like disordered open network structure at intermediate temperature. We further discuss t  ...[more]

Similar Datasets

| S-EPMC9597860 | biostudies-literature
2019-07-31 | GSE128155 | GEO
| PRJEB28595 | ENA
| S-EPMC10511685 | biostudies-literature
| S-EPMC6659638 | biostudies-literature
| S-EPMC7567402 | biostudies-literature
| S-EPMC8241080 | biostudies-literature
| S-EPMC6295875 | biostudies-literature
| S-EPMC9089292 | biostudies-literature
| S-EPMC4429515 | biostudies-literature