Ontology highlight
ABSTRACT:
SUBMITTER: Fidler AF
PROVIDER: S-EPMC3976994 | biostudies-literature | 2014
REPOSITORIES: biostudies-literature
Fidler Andrew F AF Singh Ved P VP Long Phillip D PD Dahlberg Peter D PD Engel Gregory S GS
Nature communications 20140101
Time-resolved ultrafast optical probes of chiral dynamics provide a new window allowing us to explore how interactions with such structured environments drive electronic dynamics. Incorporating optical activity into time-resolved spectroscopies has proven challenging because of the small signal and large achiral background. Here we demonstrate that two-dimensional electronic spectroscopy can be adapted to detect chiral signals and that these signals reveal how excitations delocalize and contract ...[more]