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Estimating PM2.5 Concentrations in Xi'an City Using a Generalized Additive Model with Multi-Source Monitoring Data.

ABSTRACT: Particulate matter with an aerodynamic diameter <2.5 μm (PM2.5) represents a severe environmental problem and is of negative impact on human health. Xi'an City, with a population of 6.5 million, is among the highest concentrations of PM2.5 in China. In 2013, in total, there were 191 days in Xi'an City on which PM2.5 concentrations were greater than 100 μg/m3. Recently, a few studies have explored the potential causes of high PM2.5 concentration using remote sensing data such as the MODIS aerosol optical thickness (AOT) product. Linear regression is a commonly used method to find statistical relationships among PM2.5 concentrations and other pollutants, including CO, NO2, SO2, and O3, which can be indicative of emission sources. The relationships of these variables, however, are usually complicated and non-linear. Therefore, a generalized additive model (GAM) is used to estimate the statistical relationships between potential variables and PM2.5 concentrations. This model contains linear functions of SO2 and CO, univariate smoothing non-linear functions of NO2, O3, AOT and temperature, and bivariate smoothing non-linear functions of location and wind variables. The model can explain 69.50% of PM2.5 concentrations, with R2 = 0.691, which improves the result of a stepwise linear regression (R2 = 0.582) by 18.73%. The two most significant variables, CO concentration and AOT, represent 20.65% and 19.54% of the deviance, respectively, while the three other gas-phase concentrations, SO2, NO2, and O3 account for 10.88% of the total deviance. These results show that in Xi'an City, the traffic and other industrial emissions are the primary source of PM2.5. Temperature, location, and wind variables also non-linearly related with PM2.5.

SUBMITTER: Song YZ

PROVIDER: S-EPMC4634950 | biostudies-literature |

REPOSITORIES: biostudies-literature

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Project description:Predicting long-term spatiotemporal characteristics of fine particulate matter (PM2.5) is important in China to understand historical levels of PM2.5, to support health effects research of both long-term and short-term exposures to PM2.5, and to evaluate the efficacy of air pollution control policies. Satellite-retrieved aerosol optical depth (AOD) provides a unique opportunity to characterize the long-term trends of ground-level PM2.5 at high spatial resolution. However, the missing rate of AOD in Northeastern China (NEC) is very high, especially in winter, and challenges the accuracy of long-term predictions of PM2.5 if left unresolved. Using random forest algorithms, this study developed a gap-filling approach combing satellite AOD, meteorological data, land use parameters, population and visibility in the NEC during 2005-2016. The model, including all predictors, combined with a model without AOD was able to fill the gap of PM2.5 predictions caused by missing AOD at 1-km resolution. The R2 (RMSE) of the full-coverage predictions was 0.81 (18.5 μg/m3) at the daily level. Gap-filled PM2.5 predictions on days with missing AOD reduced the relative prediction error from 28% to 2.5% in winter. The leave-one-year-out-cross-validation R2 (RMSE) of the full-coverage predictions was 0.65 (16.3 μg/m3) at the monthly level, indicating relatively high accuracy of predicted historical PM2.5 concentrations. Our results suggested that AOD helped increase the reliability of historical PM2.5 prediction when ground PM2.5 measurements were unavailable, even though predictions from the AOD model only accounted for approximate 37% of the whole dataset. Predicted PM2.5 level in NEC have increased since 2005, reached its peak during 2013-2015, then saw a major decline in 2016. Our high-resolution predictions also showed a south to north gradient and many pollution hot spots in the city clusters surrounding provincial capitals, as well as within large cities. Overall, by combining predictions from the AOD model with higher accuracy and predictions from the non-AOD model to achieve full coverage, our modeling approach could produce long-term, full-coverage historical PM2.5 levels in high-latitude areas in China, despite the widespread and persistent AOD missingness.

Project description:IntroductionRecent cohort studies have used exposure prediction models to estimate the association between long-term residential concentrations of fine particulate matter (PM2.5) and health. Because these prediction models rely on PM2.5 monitoring data, predictions for times before extensive spatial monitoring present a challenge to understanding long-term exposure effects. The U.S. Environmental Protection Agency (EPA) Federal Reference Method (FRM) network for PM2.5 was established in 1999.ObjectivesWe evaluated a novel statistical approach to produce high-quality exposure predictions from 1980 through 2010 in the continental United States for epidemiological applications.MethodsWe developed spatio-temporal prediction models using geographic predictors and annual average PM2.5 data from 1999 through 2010 from the FRM and the Interagency Monitoring of Protected Visual Environments (IMPROVE) networks. Temporal trends before 1999 were estimated by using a) extrapolation based on PM2.5 data in FRM/IMPROVE, b) PM2.5 sulfate data in the Clean Air Status and Trends Network, and c) visibility data across the Weather Bureau Army Navy network. We validated the models using PM2.5 data collected before 1999 from IMPROVE, California Air Resources Board dichotomous sampler monitoring (CARB dichot), the Children's Health Study (CHS), and the Inhalable Particulate Network (IPN).ResultsIn our validation using pre-1999 data, the prediction model performed well across three trend estimation approaches when validated using IMPROVE and CHS data (R2 = 0.84-0.91) with lower R2 values in early years. Model performance using CARB dichot and IPN data was worse (R2 = 0.00-0.85) most likely because of fewer monitoring sites and inconsistent sampling methods.ConclusionsOur prediction modeling approach will allow health effects estimation associated with long-term exposures to PM2.5 over extended time periods ? 30 years. Citation: Kim SY, Olives C, Sheppard L, Sampson PD, Larson TV, Keller JP, Kaufman JD. 2017. Historical prediction modeling approach for estimating long-term concentrations of PM2.5 in cohort studies before the 1999 implementation of widespread monitoring. Environ Health Perspect 125:38-46;?http://dx.doi.org/10.1289/EHP131.

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Estimating PM2.5 Concentrations in Xi'an City Using a Generalized Additive Model with Multi-Source Monitoring Data.

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