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Integration of metal-organic frameworks into an electrochemical dielectric thin film for electronic applications.


ABSTRACT: The integration of porous metal-organic frameworks onto the surface of materials, for use as functional devices, is currently emerging as a promising approach for gas sensing and flexible displays. However, research focused on potential applications in electronic devices is in its infancy. Here we present a facile strategy by which interpenetrated, crystalline metal-organic framework films are deposited onto conductive metal-plate anodes via in situ temperature-controlled electrochemical assembly. The nanostructure of the surface as well as the thickness and uniformity of the film are well controlled. More importantly, the resulting films exhibit enhanced dielectric properties compared to traditional inorganic or organic gate dielectrics. This study demonstrates the successful implementation of the rational design of metal-organic framework thin films on conductive supports with high-performance dielectric properties.

SUBMITTER: Li WJ 

PROVIDER: S-EPMC4906389 | biostudies-literature | 2016 Jun

REPOSITORIES: biostudies-literature

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Integration of metal-organic frameworks into an electrochemical dielectric thin film for electronic applications.

Li Wei-Jin WJ   Liu Juan J   Sun Zhi-Hua ZH   Liu Tian-Fu TF   Lü Jian J   Gao Shui-Ying SY   He Chao C   Cao Rong R   Luo Jun-Hua JH  

Nature communications 20160610


The integration of porous metal-organic frameworks onto the surface of materials, for use as functional devices, is currently emerging as a promising approach for gas sensing and flexible displays. However, research focused on potential applications in electronic devices is in its infancy. Here we present a facile strategy by which interpenetrated, crystalline metal-organic framework films are deposited onto conductive metal-plate anodes via in situ temperature-controlled electrochemical assembl  ...[more]

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