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Hybrid Multilayered Plasmonic Nanostars for Coherent Random Lasing.

ABSTRACT: Here, we report that hybrid multilayered plasmonic nanostars can be universally used as feedback agents for coherent random lasing in polar or nonpolar solutions containing gain material. We show that silver-enhancement of gold nanostars reduces the pumping threshold for coherent random lasing substantially for both a typical dye (R6G) and a typical fluorescent polymer (MEH-PPV). Further, we reveal that the lasing intensity and pumping threshold of random lasers based on silver-enhanced gold nanostars are not influenced by the silica coating, in contrast to gold nanostar-based random lasers, where silica-coated gold nanostars support only amplified spontaneous emission but no coherent random lasing.

SUBMITTER: Munkhbat B

PROVIDER: S-EPMC5075942 | biostudies-literature | 2016 Oct

REPOSITORIES: biostudies-literature

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Hybrid Multilayered Plasmonic Nanostars for Coherent Random Lasing.

Munkhbat Battulga B Ziegler Johannes J Pöhl Hannes H Wörister Christian C Sivun Dmitry D Scharber Markus C MC Klar Thomas A TA Hrelescu Calin C

The journal of physical chemistry. C, Nanomaterials and interfaces 20161004 41

Here, we report that hybrid multilayered plasmonic nanostars can be universally used as feedback agents for coherent random lasing in polar or nonpolar solutions containing gain material. We show that silver-enhancement of gold nanostars reduces the pumping threshold for coherent random lasing substantially for both a typical dye (R6G) and a typical fluorescent polymer (MEH-PPV). Further, we reveal that the lasing intensity and pumping threshold of random lasers based on silver-enhanced gold nan ...[more]

PMID: 27795752

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