Design principles for nonequilibrium self-assembly.
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ABSTRACT:
SUBMITTER: Nguyen M
PROVIDER: S-EPMC5167149 | biostudies-literature | 2016 Dec
REPOSITORIES: biostudies-literature
Publications
Design principles for nonequilibrium self-assembly.
Nguyen Michael M Vaikuntanathan Suriyanarayanan S
Proceedings of the National Academy of Sciences of the United States of America 20161122 50
We consider an important class of self-assembly problems, and using the formalism of stochastic thermodynamics, we derive a set of design principles for growing controlled assemblies far from equilibrium. The design principles constrain the set of configurations that can be obtained under nonequilibrium conditions. Our central result provides intuition for how equilibrium self-assembly landscapes are modified under finite nonequilibrium drive. ...[more]
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