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Time-reversal symmetry breaking hidden order in Sr₂(Ir,Rh)O₄.

ABSTRACT: Layered 5d transition iridium oxides, Sr₂(Ir,Rh)O₄, are described as unconventional Mott insulators with strong spin-orbit coupling. The undoped compound, Sr₂IrO₄, is a nearly ideal two-dimensional pseudospin-1/2 Heisenberg antiferromagnet, similarly to the insulating parent compound of high-temperature superconducting copper oxides. Using polarized neutron diffraction, we here report a hidden magnetic order in pure and doped Sr₂(Ir,Rh)O₄, distinct from the usual antiferromagnetic pseudospin ordering. We find that time-reversal symmetry is broken while the lattice translation invariance is preserved in the hidden order phase. The onset temperature matches that of the odd-parity hidden order recently highlighted using optical second-harmonic generation experiments. The novel magnetic order and broken symmetries can be explained by the loop-current model, previously predicted for the copper oxide superconductors.

SUBMITTER: Jeong J

PROVIDER: S-EPMC5413971 | biostudies-literature |

REPOSITORIES: biostudies-literature

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