Dataset Information

Room-temperature helimagnetism in FeGe thin films.

ABSTRACT: Chiral magnets are promising materials for the realisation of high-density and low-power spintronic memory devices. For these future applications, a key requirement is the synthesis of appropriate materials in the form of thin films ordering well above room temperature. Driven by the Dzyaloshinskii-Moriya interaction, the cubic compound FeGe exhibits helimagnetism with a relatively high transition temperature of 278?K in bulk crystals. We demonstrate that this temperature can be enhanced significantly in thin films. Using x-ray scattering and ferromagnetic resonance techniques, we provide unambiguous experimental evidence for long-wavelength helimagnetic order at room temperature and magnetic properties similar to the bulk material. We obtain ? intr?=?0.0036?±?0.0003 at 310?K for the intrinsic damping parameter. We probe the dynamics of the system by means of muon-spin rotation, indicating that the ground state is reached via a freezing out of slow dynamics. Our work paves the way towards the fabrication of thin films of chiral magnets that host certain spin whirls, so-called skyrmions, at room temperature and potentially offer integrability into modern electronics.

SUBMITTER: Zhang SL

PROVIDER: S-EPMC5427977 | biostudies-literature | 2017 Mar

REPOSITORIES: biostudies-literature

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Room-temperature helimagnetism in FeGe thin films.

Zhang S L SL Stasinopoulos I I Lancaster T T Xiao F F Bauer A A Rucker F F Baker A A AA Figueroa A I AI Salman Z Z Pratt F L FL Blundell S J SJ Prokscha T T Suter A A Waizner J J Garst M M Grundler D D van der Laan G G Pfleiderer C C Hesjedal T T

Scientific reports 20170309 1

Chiral magnets are promising materials for the realisation of high-density and low-power spintronic memory devices. For these future applications, a key requirement is the synthesis of appropriate materials in the form of thin films ordering well above room temperature. Driven by the Dzyaloshinskii-Moriya interaction, the cubic compound FeGe exhibits helimagnetism with a relatively high transition temperature of 278 K in bulk crystals. We demonstrate that this temperature can be enhanced signifi ...[more]

PMID: 28273923

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Project description:The role that interfaces play in the dynamics of liquids is a fundamental scientific problem with vast importance in technological applications. From material science to biology, e.g., batteries to cell membranes, liquid properties at interfaces are frequently determinant in the nature of chemical processes. For most liquids, like water, the influence of an interface falls off on a ∼1 nm distance scale. Room temperature ionic liquids (RTILs) are a vast class of unusual liquids composed of complex cations and anions that are liquid salts at room temperature. They are unusual liquids with properties that can be finely tuned by selecting the structure of the cation and anion. RTILs are being used or developed in applications such as batteries, CO2 capture, and liquids for biological processes. Here, it is demonstrated quantitatively that the influence of an interface on RTIL properties is profoundly different from that observed in other classes of liquids. The dynamics of planar thin films of the room temperature ionic liquid, 1-butyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (BmimNTf2), were investigated using two-dimensional infrared spectroscopy (2D IR) with the CN stretch of SeCN- as the vibrational probe. The structural dynamics (spectral diffusion) of the thin films with controlled nanometer thicknesses were measured and compared to the dynamics of the bulk liquid. The samples were prepared by spin coating the RTIL, together with the vibrational probe, onto a surface functionalized with an ionic monolayer that mimics the structure of the BmimNTf2. Near-Brewster's angle reflection pump-probe geometry 2D IR facilitated the detection of the exceedingly small signals from the films, some of which were only 14 nm thick. Even in quarter micron (250 nm) thick films, the observed dynamics were much slower than those of the bulk liquid. Using a new theoretical description, the correlation length (exponential falloff of the influence of the interfaces) was found to be 28 ± 5 nm. This very long correlation length, ∼30 times greater than that of water, has major implications for the use of RTILs in devices and other applications.

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Room-temperature helimagnetism in FeGe thin films.

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Room-temperature helimagnetism in FeGe thin films.

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