Browse
Submit Data
Databases
API
Help

Dataset Information

0 Views

0 Connections

0 Citations

0 Reanalyses

0 Downloads

Omics score: 0

Photonic hypercrystals for control of light-matter interactions.

ABSTRACT: Photonic crystals (PCs) have emerged as one of the most widely used platforms for controlling light-matter interaction in solid-state systems. They rely on Bragg scattering from wavelength-sized periodic modulation in the dielectric environment for manipulating the electromagnetic field. A complementary approach to manipulate light-matter interaction is offered by artificial media known as metamaterials that rely on the average response of deep-subwavelength unit cells. Here we demonstrate a class of artificial photonic media termed "photonic hypercrystals" (PHCs) that combine the large broadband photonic density of states provided by hyperbolic metamaterials with the light-scattering efficiency of PCs. Enhanced radiative rate (20×) and light outcoupling (100×) from PHCs embedded with quantum dots is observed. Such designer photonic media with complete control over the optical properties provide a platform for broadband control of light-matter interaction.

SUBMITTER: Galfsky T

PROVIDER: S-EPMC5441758 | biostudies-literature | 2017 May

REPOSITORIES: biostudies-literature

ACCESS DATA

Json Xml

Publications

Photonic hypercrystals for control of light-matter interactions.

Galfsky Tal T Gu Jie J Narimanov Evgenii E EE Menon Vinod M VM

Proceedings of the National Academy of Sciences of the United States of America 20170501 20

Photonic crystals (PCs) have emerged as one of the most widely used platforms for controlling light-matter interaction in solid-state systems. They rely on Bragg scattering from wavelength-sized periodic modulation in the dielectric environment for manipulating the electromagnetic field. A complementary approach to manipulate light-matter interaction is offered by artificial media known as metamaterials that rely on the average response of deep-subwavelength unit cells. Here we demonstrate a cla ...[more]

PMID: 28461458

Similar Datasets

Probing and harnessing photonic Fermi arc surface states using light-matter interactions.

Project description:Fermi arcs, i.e., surface states connecting topologically distinct Weyl points, represent a paradigmatic manifestation of the topological aspects of Weyl physics. We investigate a light-matter interface based on the photonic counterpart of these states and prove that it can lead to phenomena with no analog in other setups. First, we show how to image the Fermi arcs by studying the spontaneous decay of one or many emitters coupled to the system's border. Second, we demonstrate that, exploiting the negative refraction of these modes, the Fermi arc surface states can act as a robust quantum link, enabling, e.g., the occurrence of perfect quantum state transfer between the considered emitters or the formation of highly entangled states. In addition to their fundamental interest, our findings evidence the potential offered by the photonic Fermi arc light-matter interfaces for the design of more robust quantum technologies.

| S-EPMC10413654 | biostudies-literature

Coherent control of light-matter interactions in polarization standing waves.

Project description:We experimentally demonstrate that standing waves formed by two coherent counter-propagating light waves can take a variety of forms, offering new approaches to the interrogation and control of polarization-sensitive light-matter interactions in ultrathin (subwavelength thickness) media. In contrast to familiar energy standing waves, polarization standing waves have constant electric and magnetic energy densities and a periodically varying polarization state along the wave axis. counterintuitively, anisotropic ultrathin (meta)materials can be made sensitive or insensitive to such polarization variations by adjusting their azimuthal angle.

| S-EPMC4981885 | biostudies-literature

Tailoring Two-Dimensional Matter Using Strong Light-Matter Interactions.

Project description:The shaping of matter into desired nanometric structures with on-demand functionalities can enhance the miniaturization of devices in nanotechnology. Herein, strong light-matter interaction was used as an optical lithographic tool to tailor two-dimensional (2D) matter into nanoscale architectures. We transformed 2D black phosphorus (BP) into ultrafine, well-defined, beyond-diffraction-limit nanostructures of ten times smaller size and a hundred times smaller spacing than the incident, femtosecond-pulsed light wavelength. Consequently, nanoribbons and nanocubes/cuboids scaling tens of nanometers were formed by the structured ablation along the extremely confined periodic light fields originating from modulation instability, the tailoring process of which was visualized in real time via light-coupled in situ transmission electron microscopy. The current findings on the controllable nanoscale shaping of BP will enable exotic physical phenomena and further advance the optical lithographic techniques for 2D materials.

| S-EPMC10141415 | biostudies-literature

Nanofocusing of structured light for quadrupolar light-matter interactions.

Project description:The spatial structure of an electromagnetic field can determine the characteristics of light-matter interactions. A strong gradient of light in the near field can excite dipole-forbidden atomic transitions, e.g., electric quadrupole transitions, which are rarely observed under plane-wave far-field illumination. Structured light with a higher-order orbital angular momentum state may also modulate the selection rules in which an atom can absorb two quanta of angular momentum: one from the spin and another from the spatial structure of the beam. Here, we numerically demonstrate a strong focusing of structured light with a higher-order orbital angular momentum state in the near field. A quadrupole field was confined within a gap region of several tens of nanometres in a plasmonic tetramer structure. A plasmonic crystal surrounding the tetramer structure provides a robust antenna effect, where the incident structured light can be strongly coupled to the quadrupole field in the gap region with a larger alignment tolerance. The proposed system is expected to provide a platform for light-matter interactions with strong multipolar effects.

| S-EPMC5958059 | biostudies-literature

Nanoscale light-matter interactions in atomic cladding waveguides.

Project description:Alkali vapours, such as rubidium, are being used extensively in several important fields of research such as slow and stored light nonlinear optics quantum computation, atomic clocks and magnetometers. Recently, there is a growing effort towards miniaturizing traditional centimetre-size vapour cells. Owing to the significant reduction in device dimensions, light-matter interactions are greatly enhanced, enabling new functionalities due to the low power threshold needed for nonlinear interactions. Here, taking advantage of the mature platform of silicon photonics, we construct an efficient and flexible platform for tailored light-vapour interactions on a chip. Specifically, we demonstrate light-matter interactions in an atomic cladding waveguide, consisting of a silicon nitride nano-waveguide core with a rubidium vapour cladding. We observe the efficient interaction of the electromagnetic guided mode with the rubidium cladding and show that due to the high confinement of the optical mode, the rubidium absorption saturates at powers in the nanowatt regime.

| S-EPMC3615375 | biostudies-literature

Coherent poly propagation materials with 3-dimensional photonic control over visible light.

Project description:The purpose of the present research was to identify and examine materials demonstrating a previously undiscovered property of coherent poly propagation (CPP). The materials were amorphous silicates as natural precious opals. CPP enabled three-dimensional photonic control over mono and polychromatic visible light wavelengths. CPP caused coherent diffraction of incident poly and monochromatic light. Apart from the iconic play-of-color of precious opal, CPP specimens demonstrated diffractive photonic demultiplexing and/or upconversion and/or downconversion of incident light with strong photonic coherence such that the shape of the incident light source was propagated over three dimensions over multiple visible frequencies. CPP events manifested as each specimen was rocked under the incident light. Additionally, the specimens demonstrated atypical control over internally reflected and transmitted light. The specimens applied axial rotational symmetry over the incident light. Amorphous materials would be expected to exert no symmetry control. CPP and rotational properties occurred in isolation from exogenous thermal, photonic and electrical influences. Furthermore, several non-destructive analytical instruments were employed, such as: spectrophotometer, polariscope and refractometer. The analytical methods revealed unusual behaviors of these specimens. The application of materials demonstrating three-dimensional photonic control will have far-reaching implications for many industries, including: photonic wavelength demultiplexing, fiber optics, imaging, microscopy, projections, security, cryptography, computers and communications.

| S-EPMC6797174 | biostudies-literature

Transition Metal Dichalcogenide Dimer Nanoantennas for Tailored Light-Matter Interactions.

Project description:Transition metal dichalcogenides have emerged as promising materials for nanophotonic resonators because of their large refractive index, low absorption within a large portion of the visible spectrum, and compatibility with a wide range of substrates. Herein, we use these properties to fabricate WS2 double-pillar nanoantennas in a variety of geometries enabled by the anisotropy in the crystal structure. Using dark-field spectroscopy, we reveal multiple Mie resonances, to which we couple WSe2 monolayer photoluminescence and achieve Purcell enhancement and an increased fluorescence by factors up to 240 for dimer gaps of 150 nm. We introduce postfabrication atomic force microscope repositioning and rotation of dimer nanoantennas, achieving gaps as small as 10 ± 5 nm, which enables a host of potential applications, including strong Purcell enhancement of single-photon emitters and optical trapping, which we study in simulations. Our findings highlight the advantages of using transition metal dichalcogenides for nanophotonics by exploring applications enabled by their properties.

| S-EPMC9047003 | biostudies-literature

Voltage-Controlled Switching of Strong Light-Matter Interactions using Liquid Crystals.

Project description:We experimentally demonstrate a fine control over the coupling strength of vibrational light-matter hybrid states by controlling the orientation of a nematic liquid crystal. Through an external voltage, the liquid crystal is seamlessly switched between two orthogonal directions. Using these features, for the first time, we demonstrate electrical switching and increased Rabi splitting through transition dipole moment alignment. The C-Nstr vibration on the liquid crystal molecule is coupled to a cavity mode, and FT-IR is used to probe the formed vibropolaritonic states. A switching ratio of the Rabi splitting of 1.78 is demonstrated between the parallel and the perpendicular orientation. Furthermore, the orientational order increases the Rabi splitting by 41?% as compared to an isotropic liquid. Finally, by examining the influence of molecular alignment on the Rabi splitting, the scalar product used in theoretical modeling between light and matter in the strong coupling regime is verified.

| S-EPMC5814857 | biostudies-other

Super-resolution imaging of light-matter interactions near single semiconductor nanowires.

Project description:Nanophotonics is becoming invaluable for an expanding range of applications, from controlling the spontaneous emission rate and the directionality of quantum emitters, to reducing material requirements of solar cells by an order of magnitude. These effects are highly dependent on the near field of the nanostructure, which constitutes the evanescent fields from propagating and resonant localized modes. Although the interactions between quantum emitters and nanophotonic structures are increasingly well understood theoretically, directly imaging these interactions experimentally remains challenging. Here we demonstrate a photoactivated localization microscopy-based technique to image emitter-nanostructure interactions. For a 75?nm diameter silicon nanowire, we directly observe a confluence of emission rate enhancement, directivity modification and guided mode excitation, with strong interaction at scales up to 13 times the nanowire diameter. Furthermore, through analytical modelling we distinguish the relative contribution of these effects, as well as their dependence on emitter orientation.

| S-EPMC5187462 | biostudies-literature

Selective manipulation of electronically excited states through strong light-matter interactions.

Project description:Strong coupling between light and matter leads to the spontaneous formation of hybrid light-matter states, having different energies than the uncoupled states. This opens up for new ways of modifying the energy landscape of molecules without changing their atoms or structure. Heavy metal-free organic light emitting diodes (OLED) use reversed intersystem crossing (RISC) to harvest light from excited triplet states. This is a slow process, thus increasing the rate of RISC could potentially enhance OLED performance. Here we demonstrate selective coupling of the excited singlet state of Erythrosine B without perturbing the energy level of a nearby triplet state. The coupling reduces the triplet-singlet energy gap, leading to a four-time enhancement of the triplet decay rate, most likely due to an enhanced rate of RISC. Furthermore, we anticipate that strong coupling can be used to create energy-inverted molecular systems having a singlet ground and lowest excited state.

| S-EPMC5995866 | biostudies-literature

OmicsDI is part of the ELIXIR infrastructure

OmicsDI is an Elixir interoperability service. Learn more ›

Tweets

OmicsDI Databases

PRIDE
PeptideAtlas
MassIVE
JPOST Repository
Physiome Model Repository

EGA
EVA
ENA
LINCS
PAXDB
Cell Collective

MetaboLights
Metabolomics Workbench
MetabolomeExpress
GNPS
BioModels
FAIRDOMHub

ArrayExpress
dbGaP
ExpressionAtlas
GEO
NODE

Information

Databases
Help
API
Contact us
Code on GitHub
Terms of use
Submit Data