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Topologically enabled optical nanomotors.

ABSTRACT: Shaping the topology of light, by way of spin or orbital angular momentum engineering, is a powerful tool to manipulate matter on the nanoscale. Conventionally, such methods focus on shaping the incident beam of light and not the full interaction between the light and the object to be manipulated. We theoretically show that tailoring the topology of the phase space of the light particle interaction is a fundamentally more versatile approach, enabling dynamics that may not be achievable by shaping of the light alone. In this manner, we find that optically asymmetric (Janus) particles can become stable nanoscale motors even in a light field with zero angular momentum. These precessing steady states arise from topologically protected anticrossing behavior of the vortices of the optical torque vector field. Furthermore, by varying the wavelength of the incident light, we can control the number, orientations, and the stability of the spinning states. These results show that the combination of phase-space topology and particle asymmetry can provide a powerful degree of freedom in designing nanoparticles for optimal external manipulation in a range of nano-optomechanical applications.

SUBMITTER: Ilic O

PROVIDER: S-EPMC5493414 | biostudies-literature | 2017 Jun

REPOSITORIES: biostudies-literature

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Topologically enabled optical nanomotors.

Ilic Ognjen O Kaminer Ido I Zhen Bo B Miller Owen D OD Buljan Hrvoje H Soljačić Marin M Soljačić Marin M

Science advances 20170630 6

Shaping the topology of light, by way of spin or orbital angular momentum engineering, is a powerful tool to manipulate matter on the nanoscale. Conventionally, such methods focus on shaping the incident beam of light and not the full interaction between the light and the object to be manipulated. We theoretically show that tailoring the topology of the phase space of the light particle interaction is a fundamentally more versatile approach, enabling dynamics that may not be achievable by shapin ...[more]

PMID: 28695194

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Project description:Enabled by the proliferation of nanoscale fabrication techniques required to create spatially-repeating, sub-wavelength structures to manipulate the behavior of visible-wavelength radiation, optical metamaterials are of increasing interest. Here we develop and characterize a chemical sensing approach based on electrochemical tuning of the optical response function of large-area, inexpensive nanoaperture metamaterials at visible and near-IR wavelengths. Nanosphere lithography is used to create an ordered array of sub-wavelength apertures in a Au film. The spacing of these apertures is established during fabrication, based on the size of the polystyrene nanospheres. Tunable shifts in the transmission spectrum can be produced post-fabrication by electrodeposition of a dissimilar metal, Ag, using the nanoaperture film as one electrode in a 2-electrode closed bipolar electrochemical (CBE) cell, altering hole size, film thickness, and film composition while maintaining hole spacing dictated by the original pattern. Optical transmission spectra acquired under galvanostatic conditions can be expressed as a linear combination of the initial and final (saturated) spectra, and the resulting response function exhibits a sigmoidal response with respect to the amount of charge (or metal) deposited. This architecture is then used to perform optical coulometry of model analytes in a CBE-based analyte-reporter dual cell device, thus expanding the capability of CBE-based sensors. Increasing the exposed electrode area of the analyte cell increases the response of the device, while modifying the circuit resistance alters the balance between sensitivity and dynamic range. These tunable nanoaperture metamaterials exhibit enhanced sensitivity compared to CBE electrochromic reporter cells to the μM to nM concentration range, suggesting further avenues for development of CBE-based chemical sensors as well as application to inexpensive, point-of-care diagnostic devices.

Dataset Information

Topologically enabled optical nanomotors.

Publications

Topologically enabled optical nanomotors.

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