Browse
Submit Data
Databases
API
Help

Dataset Information

12 Views

0 Connections

0 Citations

0 Reanalyses

0 Downloads

Omics score: 0

Photonic Effects for Magnetic Dipole Transitions.

ABSTRACT: The radiative transition probability is a fundamental property for optical transitions. Extensive research, theoretical and experimental, has been conducted to establish the relation between the photonic environment and electric dipole (ED) transition probabilities. Recent work shows that the nanocrystal (NC)-cavity model accurately describes the influence of the refractive index n on ED transition rates for emitters in NCs. For magnetic dipole (MD) transitions, theory predicts a simple n3 dependence. However, experimental evidence is sparse and difficult to obtain. Here we report Eu3+-(with distinct ED+MD transitions) and Gd3+-(MD transitions) doped ?-NaYF4 NC model systems to probe the influence of n on ED and MD transition probabilities through luminescence lifetime and ED/MD intensity ratio measurements. The results provide strong experimental evidence for an n3 dependence of MD transition probabilities. This insight is important for understanding and controlling the variation of spectral distribution in emission spectra by photonic effects.

SUBMITTER: Wang Z

PROVIDER: S-EPMC5724029 | biostudies-literature | 2017 Dec

REPOSITORIES: biostudies-literature

ACCESS DATA

Json Xml

Publications

Photonic Effects for Magnetic Dipole Transitions.

Wang Zijun Z Senden Tim T Meijerink Andries A

The journal of physical chemistry letters 20171108 23

The radiative transition probability is a fundamental property for optical transitions. Extensive research, theoretical and experimental, has been conducted to establish the relation between the photonic environment and electric dipole (ED) transition probabilities. Recent work shows that the nanocrystal (NC)-cavity model accurately describes the influence of the refractive index n on ED transition rates for emitters in NCs. For magnetic dipole (MD) transitions, theory predicts a simple n<sup>3< ...[more]

PMID: 29111761

Similar Datasets

Low loss photonic nanocavity via dark magnetic dipole resonant mode near metal.

Project description:The dielectric-semiconductor-dielectric-metal 4 layered structure is a well-established configuration to support TM hybrid plasmonic modes, which have demonstrated significant advantages over pure photonic modes in structures without metal to achieve low loss resonant cavities at sub-diffraction limited volumes. The photonic modes with TE characteristics supported by the same 4 layered structure, on the other hand, are less studied. Here we show that a low loss photonic mode with TE01 characteristics exists in the dielectric-semiconductor-dielectric-metal 4 layered structure if a truncated cylindrical disk is chosen as the semiconductor core. This mode exhibits the lowest cavity loss among all resonant modes, including both pure photonic and hybrid plasmonic modes, at cavity radius <150?nm and within the wavelength range 620?nm to 685?nm, with a footprint ~0.83 (?/2neff)2, physical size ~0.47 (?/2neff)3 and a mode volume down to 0.3 (?/2neff)3. The low cavity loss of this TE01 mode is attributed to its substantially reduced radiation loss to the far field by the creation of image charges through the metal response. Because of the low mode penetration in the metal, this photonic mode show equally low cavity loss near industry relevant metals such as Cu. Our study demonstrates an alternative to hybrid plamonic modes and metallo-dielectric modes to achieve low loss cavities with extremely small footprints.

| S-EPMC6242897 | biostudies-other

Unidirectional propagation of the Bloch surface wave excited by the spinning magnetic dipole in two-dimensional photonic crystal slab.

Project description:The photonic spin Hall effect (PSHE) can be realized in a photonic crystal (PC) slab, that is, the unidirectional Bloch surface wave can propagate along the surface of the PC slab under the excitation of elliptical polarized magnetic dipole. It is further proved that PSHE is caused by the interference of the component surface waves excited by the different components of the incident light, which is the so called component wave interference (CWI) theory. In addition, we also find that the spin of the surface wave oscillates periodically in space, and the oscillation period is a unit cell. In a unit cell, the average spin keeps the spin orbit locked. The results show that the spin separation can also be modulated by the position and the polarization state of the magnetic dipole.

| S-EPMC8445978 | biostudies-literature

Mantle cloaking due to ideal magnetic dipole scattering.

Project description:One of the most exciting applications of metaparticles and metasurfaces consists in the magnetic light excitation. However, the principal limitation is due to parasitic extra multipoles of electric family excited in magnetic dipole meta-particles characterized by a radiating nature and corresponding radiating losses. In this paper, we propose the "ideal magnetic dipole" with suppressed additional multipoles except of magnetic dipole moment in the scattered field from a cylindrical object by using mantle cloaking based on metasurface and on anapole concept. The considered metasurface consists of a periodic width modulated microstrip line, with a sinusoidally shaped profile unit cell printed on a dielectric substrate.

| S-EPMC7016144 | biostudies-literature

Bright magnetic dipole radiation from two-dimensional lead-halide perovskites.

Project description:Light-matter interactions in semiconductors are uniformly treated within the electric dipole approximation; multipolar interactions are considered "forbidden." We experimentally demonstrate that this approximation inadequately describes light emission in two-dimensional (2D) hybrid organic-inorganic perovskites (HOIPs), solution processable semiconductors with promising optoelectronic properties. By exploiting the highly oriented crystal structure, we use energy-momentum spectroscopies to demonstrate that an exciton-like sideband in 2D HOIPs exhibits a multipolar radiation pattern with highly directed emission. Electromagnetic and quantum-mechanical analyses indicate that this emission originates from an out-of-plane magnetic dipole transition arising from the 2D character of electronic states. Symmetry arguments and temperature-dependent measurements suggest a dynamic symmetry-breaking mechanism that is active over a broad temperature range. These results challenge the paradigm of electric dipole-dominated light-matter interactions in optoelectronic materials, provide new perspectives on the origins of unexpected sideband emission in HOIPs, and tease the possibility of metamaterial-like scattering phenomena at the quantum-mechanical level.

| S-EPMC7007269 | biostudies-literature

The dipole moment of the spin density as a local indicator for phase transitions.

Project description:The intra-atomic magnetic dipole moment - frequently called ?Tz? term - plays an important role in the determination of spin magnetic moments by x-ray absorption spectroscopy for systems with nonspherical spin density distributions. In this work, we present the dipole moment as a sensitive monitor to changes in the electronic structure in the vicinity of a phase transiton. In particular, we studied the dipole moment at the Fe(2+) and Fe(3+) sites of magnetite as an indicator for the Verwey transition by a combination of x-ray magnetic circular dichroism and density functional theory. Our experimental results prove that there exists a local change in the electronic structure at temperatures above the Verwey transition correlated to the known spin reorientation. Furthermore, it is shown that measurement of the dipole moment is a powerful tool to observe this transition in small magnetite nanoparticles for which it is usually screened by blocking effects in classical magnetometry.

| S-EPMC4104392 | biostudies-literature

Gyre-driven decay of the Earth's magnetic dipole.

Project description:Direct observations indicate that the magnitude of the Earth's magnetic axial dipole has decreased over the past 175 years; it is now 9% weaker than it was in 1840. Here we show how the rate of dipole decay may be controlled by a planetary-scale gyre in the liquid metal outer core. The gyre's meridional limbs on average transport normal polarity magnetic flux equatorward and reverse polarity flux poleward. Asymmetry in the geomagnetic field, due to the South Atlantic Anomaly, is essential to the proposed mechanism. We find that meridional flux advection accounts for the majority of the dipole decay since 1840, especially during times of rapid decline, with magnetic diffusion making an almost steady contribution generally of smaller magnitude. Based on the morphology of the present field, and the persistent nature of the gyre, the current episode of dipole decay looks set to continue, at least for the next few decades.

| S-EPMC4737809 | biostudies-other

Radiated and guided optical waves of a magnetic dipole-nanofiber system.

Project description:Nanophotonics-photonic structures with subwavelength features-allow accessing high intensity and localized electromagnetic field and hence is an ideal platform for investigating and exploiting strong lightmatter interaction. In particular, such a strong light-matter interaction requires investigating the interaction of a magnetic dipole with the electromagnetic field- a less-explored topic, which has usually been ignored within the framework of electric dipole approximation. Motivated by recent advances in the emerging field of multipolar nanophotonics, here we develop an analytical model that provides a new insight into analyzing a magnetic dipole and a nanofiber. This method enables us to examine the effect of second term in the multipolar expansion of light-matter interaction, magnetic dipole approximation, with individual guided and radiation modes of the nanofiber. This is a critical key in developing nanophotonic integrated devices based on magnetic nature of light for super-imaging, biosensing, and optical computing.

| S-EPMC6401418 | biostudies-literature

Dynamic Nonlinear Image Tuning through Magnetic Dipole Quasi-BIC Ultrathin Resonators.

Project description:Dynamical tuning of the nonlinear optical wavefront allows for a specific spectral response of predefined profiles, enabling various applications of nonlinear nanophotonics. This study experimentally demonstrates the dynamical switching of images generated by an ultrathin silicon nonlinear metasurface supporting a high-quality leaky mode, which is formed by partially breaking a bound-state-in-the-continuum (BIC) generated by the collective magnetic dipole (MD) resonance excited in the subdiffractive periodic systems. Such a quasi-BIC MD state can be excited directly under normal plane wave incidence and leads to a strong near-field enhancement to further boost the nonlinear process, resulting in a 500-fold enhancement of the third-harmonic emission experimentally. Due to sharp spectral features and asymmetry of the unit cell, it allows for effective tailoring of the nonlinear emissions over spectral or polarization responses. Dynamical nonlinear image tuning is experimentally demonstarted via polarization and wavelength control. The results pave the way for nanophotonics applications such as tunable displays, nonlinear holograms, tunable nanolaser, and ultrathin nonlinear nanodevices with various functionalities.

| S-EPMC6685498 | biostudies-literature

Helix Dipole and Membrane Electrostatics Delineate Conformational Transitions in the Self-Assembly of Amyloidogenic Peptides.

Project description:The self-assembly of amyloidogenic peptides on membrane surfaces is associated with the death of neurons and β-cells in Alzheimer's disease and type 2 diabetes, respectively. The early events of self-assembly in vivo are not known, but there is increasing evidence for the importance of the α-helix. To test the hypothesis that electrostatic interactions involving the helix dipole play a key role in membrane-mediated peptide self-assembly, we studied IAPP[11-25(S20G)-NH2] (R11LANFLVHSGNNFGA25-NH2), which under certain conditions self-assembles in hydro to form β-sheet assemblies through an α-helix-containing intermediate. In the presence of small unilamellar vesicles composed solely of zwitterionic lipids, the peptide does not self-assemble presumably because of the absence of stabilizing electrostatic interactions between the membrane surface and the helix dipole. In the presence of vesicles composed solely of anionic lipids, the peptide forms a long-lived α-helix presumably stabilized by dipole-dipole interactions between adjacent helix dipoles. This helix represents a kinetic trap that inhibits β-sheet formation. Intriguingly, when the amount of anionic lipids was decreased to mimic the ratio of zwitterionic and anionic lipids in cells, the α-helix was short-lived and underwent an α-helix to β-sheet conformational transition. Our work suggests that the helix dipole and membrane electrostatics delineate the conformational transitions occurring along the self-assembly pathway to the amyloid.

| S-EPMC8095063 | biostudies-literature

Tunable and switchable magnetic dipole patterns in nanostructured superconductors.

Project description:Design and manipulation of magnetic moment arrays have been at the focus of studying the interesting cooperative physical phenomena in various magnetic systems. However, long-range ordered magnetic moments are rather difficult to achieve due to the excited states arising from the relatively weak exchange interactions between the localized moments. Here, using a nanostructured superconductor, we investigate a perfectly ordered magnetic dipole pattern with the magnetic poles having the same distribution as the magnetic charges in an artificial spin ice. The magnetic states can simply be switched on/off by applying a current flowing through nanopatterned area. Moreover, by coupling magnetic dipoles with the pinned vortex lattice, we are able to erase the positive/negative poles, resulting in a magnetic dipole pattern of only one polarity, analogous to the recently predicted vortex ice. These switchable and tunable magnetic dipole patterns open pathways for the study of exotic ordering phenomena in magnetic systems.

| S-EPMC6030140 | biostudies-other

OmicsDI is part of the ELIXIR infrastructure

OmicsDI is an Elixir interoperability service. Learn more ›

OmicsDI Databases

PRIDE
PeptideAtlas
MassIVE
JPOST Repository
Physiome Model Repository

EGA
EVA
ENA
LINCS
PAXDB
Cell Collective

MetaboLights
Metabolomics Workbench
MetabolomeExpress
GNPS
BioModels
FAIRDOMHub

ArrayExpress
dbGaP
ExpressionAtlas
GEO
NODE

Information

Databases
Help
API
Contact us
Code on GitHub
Terms of use
Submit Data