Dataset Information

A hybrid model for spatially and temporally resolved ozone exposures in the continental United States.

ABSTRACT: Ground-level ozone is an important atmospheric oxidant, which exhibits considerable spatial and temporal variability in its concentration level. Existing modeling approaches for ground-level ozone include chemical transport models, land-use regression, Kriging, and data fusion of chemical transport models with monitoring data. Each of these methods has both strengths and weaknesses. Combining those complementary approaches could improve model performance. Meanwhile, satellite-based total column ozone, combined with ozone vertical profile, is another potential input. The authors propose a hybrid model that integrates the above variables to achieve spatially and temporally resolved exposure assessments for ground-level ozone. The authors used a neural network for its capacity to model interactions and nonlinearity. Convolutional layers, which use convolution kernels to aggregate nearby information, were added to the neural network to account for spatial and temporal autocorrelation. The authors trained the model with the Air Quality System (AQS) 8-hr daily maximum ozone in the continental United States from 2000 to 2012 and tested it with left out monitoring sites. Cross-validated R² on the left out monitoring sites ranged from 0.74 to 0.80 (mean 0.76) for predictions on 1 km × 1 km grid cells, which indicates good model performance. Model performance remains good even at low ozone concentrations. The prediction results facilitate epidemiological studies to assess the health effect of ozone in the long term and the short term.

Implications

Ozone monitors do not provide full data coverage over the United States, which is an obstacle to assess the health effect of ozone when monitoring data are not available. This paper used a hybrid approach to combine satellite-based ozone measurements, chemical transport model simulations, land-use terms, and other auxiliary variables to obtain spatially and temporally resolved ground-level ozone estimation.

SUBMITTER: Di Q

PROVIDER: S-EPMC5741295 | biostudies-literature | 2017 Jan

REPOSITORIES: biostudies-literature

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Publications

A hybrid model for spatially and temporally resolved ozone exposures in the continental United States.

Di Qian Q Rowland Sebastian S Koutrakis Petros P Schwartz Joel J

Journal of the Air & Waste Management Association (1995) 20170101 1

Ground-level ozone is an important atmospheric oxidant, which exhibits considerable spatial and temporal variability in its concentration level. Existing modeling approaches for ground-level ozone include chemical transport models, land-use regression, Kriging, and data fusion of chemical transport models with monitoring data. Each of these methods has both strengths and weaknesses. Combining those complementary approaches could improve model performance. Meanwhile, satellite-based total column ...[more]

PMID: 27332675

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Project description:This study analyzes simulated regional-scale ozone burdens both near the surface and aloft, estimates process contributions to these burdens, and calculates the sensitivity of the simulated regional-scale ozone burden to several key model inputs with a particular emphasis on boundary conditions derived from hemispheric or global-scale models. The Community Multiscale Air Quality (CMAQ) model simulations supporting this analysis were performed over the continental US for the year 2010 within the context of the Air Quality Model Evaluation International Initiative (AQMEII) and Task Force on Hemispheric Transport of Air Pollution (TF-HTAP) activities. CMAQ process analysis (PA) results highlight the dominant role of horizontal and vertical advection on the ozone burden in the mid-to-upper troposphere and lower stratosphere. Vertical mixing, including mixing by convective clouds, couples fluctuations in free-tropospheric ozone to ozone in lower layers. Hypothetical bounding scenarios were performed to quantify the effects of emissions, boundary conditions, and ozone dry deposition on the simulated ozone burden. Analysis of these simulations confirms that the characterization of ozone outside the regional-scale modeling domain can have a profound impact on simulated regional-scale ozone. This was further investigated by using data from four hemispheric or global modeling systems (Chemistry - Integrated Forecasting Model (C-IFS), CMAQ extended for hemispheric applications (H-CMAQ), the Goddard Earth Observing System model coupled to chemistry (GEOS-Chem), and AM3) to derive alternate boundary conditions for the regional-scale CMAQ simulations. The regional-scale CMAQ simulations using these four different boundary conditions showed that the largest ozone abundance in the upper layers was simulated when using boundary conditions from GEOS-Chem, followed by the simulations using C-IFS, AM3, and H-CMAQ boundary conditions, consistent with the analysis of the ozone fields from the global models along the CMAQ boundaries. Using boundary conditions from AM3 yielded higher springtime ozone columns burdens in the middle and lower troposphere compared to boundary conditions from the other models. For surface ozone, the differences between the AM3-driven CMAQ simulations and the CMAQ simulations driven by other large-scale models are especially pronounced during spring and winter where they can reach more than 10 ppb for seasonal mean ozone mixing ratios and as much as 15 ppb for domain-averaged daily maximum 8 h average ozone on individual days. In contrast, the differences between the C-IFS-, GEOS-Chem-, and H-CMAQ-driven regional-scale CMAQ simulations are typically smaller. Comparing simulated sur face ozone mixing ratios to observations and computing seasonal and regional model performance statistics revealed that boundary conditions can have a substantial impact on model performance. Further analysis showed that boundary conditions can affect model performance across the entire range of the observed distribution, although the impacts tend to be lower during summer and for the very highest observed percentiles. The results are discussed in the context of future model development and analysis opportunities.

Dataset Information

A hybrid model for spatially and temporally resolved ozone exposures in the continental United States.

Implications

Publications

A hybrid model for spatially and temporally resolved ozone exposures in the continental United States.

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