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Synthesis and photocatalytic activity of mesoporous g-C3N4/MoS2 hybrid catalysts.


ABSTRACT: The key to solving environmental and energy issues through photocatalytic technology requires highly efficient, stable and eco-friendly photocatalysts. Graphitic carbon nitride (g-C3N4) is one of the most promising candidates except for its limited photoactivity. In this work, a facile and scalable one-step method is developed to fabricate an efficient heterostructural g-C3N4 photocatalyst in situ coupled with MoS2. The strong coupling effect between the MoS2 nanosheets and g-C3N4 scaffold, numerous mesopores and enlarged specific surface area helped form an effective heterojunction. As such, the photocatalytic activity of the g-C3N4/MoS2 is more than three times higher than that of the pure g-C3N4 in the degradation of RhB under visible light irradiation. Improvement of g-C3N4/MoS2 photocatalytic performance is mainly ascribed to the effective suppression of the recombination of charge carriers.

SUBMITTER: Qi Y 

PROVIDER: S-EPMC5990742 | biostudies-literature | 2018 May

REPOSITORIES: biostudies-literature

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Synthesis and photocatalytic activity of mesoporous g-C<sub>3</sub>N<sub>4</sub>/MoS<sub>2</sub> hybrid catalysts.

Qi Yirong Y   Liang Qinghua Q   Lv Ruitao R   Shen Wanci W   Kang Feiyu F   Huang Zheng-Hong ZH  

Royal Society open science 20180516 5


The key to solving environmental and energy issues through photocatalytic technology requires highly efficient, stable and eco-friendly photocatalysts. Graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) is one of the most promising candidates except for its limited photoactivity. In this work, a facile and scalable one-step method is developed to fabricate an efficient heterostructural g-C<sub>3</sub>N<sub>4</sub> photocatalyst <i>in situ</i> coupled with MoS<sub>2</sub>. The strong couplin  ...[more]

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