Dataset Information

Analytical estimation of non-local deformation-mediated magneto-electric coupling in soft composites.

ABSTRACT: For a long time, the search for magneto-electric materials concentrated on multi-ferroics and hard-matter composites. By contrast, rather recently the exploitation of strain-mediated magneto-electric (ME) coupling in soft composites was proposed. The basic idea behind this approach is to combine the magneto- and electro-mechanical responses of composites consisting of a soft matrix carrying magnetic inclusions. Despite that such composites are straightforward to manufacture and have cheap constituents, they did not gain much attention up to now. In this contribution, we demonstrate that ME coupling induced by finite deformations could be of significant magnitude. Our approach relies on shape effects as a special non-local phenomenon in magneto- and electro-elasticity. Based on that we characterize an up to now overlooked ME coupling mechanism which purely relies on these shape effects in soft-matter-based magnetic and electric media. While soft magnetic media are commonly realized as composites, the coupling effect to be highlighted exists independently of the origin of a body's magnetic and electric properties. We show that the magnitude of the effect is indeed significant and, among ellipsoidal bodies, most pronounced for those of spherical to moderately prolate shape. Finite-element simulations are performed to assess the quality of the analytical predictions.

SUBMITTER: Rambausek M

PROVIDER: S-EPMC6127395 | biostudies-literature | 2018 Aug

REPOSITORIES: biostudies-literature

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Analytical estimation of non-local deformation-mediated magneto-electric coupling in soft composites.

Rambausek M M Keip M-A MA

Proceedings. Mathematical, physical, and engineering sciences 20180801 2216

For a long time, the search for magneto-electric materials concentrated on multi-ferroics and hard-matter composites. By contrast, rather recently the exploitation of strain-mediated magneto-electric (ME) coupling in soft composites was proposed. The basic idea behind this approach is to combine the magneto- and electro-mechanical responses of composites consisting of a soft matrix carrying magnetic inclusions. Despite that such composites are straightforward to manufacture and have cheap consti ...[more]

PMID: 30220865

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Project description:The magnetoelectric effect (ME) is an important strain mediated-phenomenon in a ferromagnetic-piezoelectric composite for a variety of sensors and signal processing devices. A bias magnetic field, in general, is essential to realize a strong ME coupling in most composites. Magnetic phases with (i) high magnetostriction for strong piezomagnetic coupling and (ii) large anisotropy field that acts as a built-in bias field are preferred so that miniature, ME composite-based devices can operate without the need for an external magnetic field. We are able to realize such a magnetic phase with a composite of (i) barium hexaferrite (BaM) with high magnetocrystalline anisotropy field and (ii) nickel ferrite (NFO) with high magnetostriction. The BNx composites, with (100 - x) wt.% of BaM and x wt.% NFO, for x = 0-100, were prepared. X-ray diffraction analysis shows that the composites did not contain any impurity phases. Scanning electron microscopy images revealed that, with an increase in NFO content, hexagonal BaM grains become prominent, leading to a large anisotropy field. The room temperature saturation magnetization showed a general increase with increasing BaM content in the composites. NFO rich composites with x ≥ 60 were found to have a large magnetostriction value of around -23 ppm, comparable to pure NFO. The anisotropy field HA of the composites, determined from magnetization and ferromagnetic resonance (FMR) measurements, increased with increasing NFO content and reached a maximum of 7.77 kOe for x = 75. The BNx composite was cut into rectangular platelets and bonded with PZT to form the bilayers. ME voltage coefficient (MEVC) measurements at low frequencies and at mechanical resonance showed strong coupling at zero bias for samples with x ≥ 33. This large in-plane HA acted as a built-in field for strong ME effects under zero external bias in the bilayers. The highest zero-bias MEVC of ~22 mV/cm Oe was obtained for BN75-PZT bilayers wherein BN75 also has the highest HA. The Bilayer of BN95-PZT showed a maximum MEVC ~992 mV/cm Oe at electromechanical resonance at 59 kHz. The use of hexaferrite-spinel ferrite composite to achieve strong zero-bias ME coupling in bilayers with PZT is significant for applications related to energy harvesting, sensors, and high frequency devices.

Dataset Information

Analytical estimation of non-local deformation-mediated magneto-electric coupling in soft composites.

Publications

Analytical estimation of non-local deformation-mediated magneto-electric coupling in soft composites.

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