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Atomic-scale strain manipulation of a charge density wave.


ABSTRACT: A charge density wave (CDW) is one of the fundamental instabilities of the Fermi surface occurring in a wide range of quantum materials. In dimensions higher than one, where Fermi surface nesting can play only a limited role, the selection of the particular wavevector and geometry of an emerging CDW should in principle be susceptible to controllable manipulation. In this work, we implement a simple method for straining materials compatible with low-temperature scanning tunneling microscopy/spectroscopy (STM/S), and use it to strain-engineer CDWs in 2H-NbSe2 Our STM/S measurements, combined with theory, reveal how small strain-induced changes in the electronic band structure and phonon dispersion lead to dramatic changes in the CDW ordering wavevector and geometry. Our work unveils the microscopic mechanism of a CDW formation in this system, and can serve as a general tool compatible with a range of spectroscopic techniques to engineer electronic states in any material where local strain or lattice symmetry breaking plays a role.

SUBMITTER: Gao S 

PROVIDER: S-EPMC6142222 | biostudies-literature | 2018 Jul

REPOSITORIES: biostudies-literature

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Atomic-scale strain manipulation of a charge density wave.

Gao Shang S   Flicker Felix F   Sankar Raman R   Zhao He H   Ren Zheng Z   Rachmilowitz Bryan B   Balachandar Sidhika S   Chou Fangcheng F   Burch Kenneth S KS   Wang Ziqiang Z   van Wezel Jasper J   Zeljkovic Ilija I  

Proceedings of the National Academy of Sciences of the United States of America 20180618 27


A charge density wave (CDW) is one of the fundamental instabilities of the Fermi surface occurring in a wide range of quantum materials. In dimensions higher than one, where Fermi surface nesting can play only a limited role, the selection of the particular wavevector and geometry of an emerging CDW should in principle be susceptible to controllable manipulation. In this work, we implement a simple method for straining materials compatible with low-temperature scanning tunneling microscopy/spect  ...[more]

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