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Effects of Interfacial Passivation on the Electrical Performance, Stability, and Contact Properties of Solution Process Based ZnO Thin Film Transistors.


ABSTRACT: This paper reports low temperature solution processed ZnO thin film transistors (TFTs), and the effects of interfacial passivation of a 4-chlorobenzoic acid (PCBA) layer on device performance. It was found that the ZnO TFTs with PCBA interfacial modification layers exhibited a higher electron mobility of 4.50 cm² V-1 s-1 compared to the pristine ZnO TFTs with a charge carrier mobility of 2.70 cm² V-1 s-1. Moreover, the ZnO TFTs with interfacial modification layers could significantly improve device shelf-life stability and bias stress stability compared to the pristine ZnO TFTs. Most importantly, interfacial modification layers could also decrease the contact potential barrier between the source/drain electrodes and the ZnO films when using high work-function metals such as Ag and Au. These results indicate that high performance TFTs can be obtained with a low temperature solution process with interfacial modification layers, which strongly implies further potential for their applications.

SUBMITTER: Wan L 

PROVIDER: S-EPMC6163572 | biostudies-literature | 2018 Sep

REPOSITORIES: biostudies-literature

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Effects of Interfacial Passivation on the Electrical Performance, Stability, and Contact Properties of Solution Process Based ZnO Thin Film Transistors.

Wan Liaojun L   He Fuchao F   Qin Yu Y   Lin Zhenhua Z   Su Jie J   Chang Jingjing J   Hao Yue Y  

Materials (Basel, Switzerland) 20180918 9


This paper reports low temperature solution processed ZnO thin film transistors (TFTs), and the effects of interfacial passivation of a 4-chlorobenzoic acid (PCBA) layer on device performance. It was found that the ZnO TFTs with PCBA interfacial modification layers exhibited a higher electron mobility of 4.50 cm² V<sup>-1</sup> s<sup>-1</sup> compared to the pristine ZnO TFTs with a charge carrier mobility of 2.70 cm² V<sup>-1</sup> s<sup>-1</sup>. Moreover, the ZnO TFTs with interfacial modific  ...[more]

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