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Double-Shelled Phosphorus and Nitrogen Codoped Carbon Nanospheres as Efficient Polysulfide Mediator for High-Performance Lithium-Sulfur Batteries.

ABSTRACT: Lithium-sulfur batteries are regarded as very promising energy storage devices due to their high energy density, low cost, and environmental friendliness; however, their insulating properties and the instability of sulfur-based electrodes impede the practical applications of Li-S batteries. Here, a versatile strategy to synthesize double-shelled nitrogen and phosphorus codoped carbon spheres (NPDSCS) as an efficient sulfur host for Li-S batteries is reported. With strong trapping, good affinity, high adsorption for polysulfides, and the bifunctional catalyzing for sulfur redox processes, the developed NPDSCS cathodes with a high S loading of 72.4% exhibit large specific discharge capacity of 1326 mAh g-1 at 0.1C, high Coulombic efficiency, good rate capability, and excellent cycling performance with a reversible capacity of 814 mAh g-1 at 1C after 500 cycles.

SUBMITTER: Wang J 

PROVIDER: S-EPMC6247042 | biostudies-literature | 2018 Nov

REPOSITORIES: biostudies-literature

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Double-Shelled Phosphorus and Nitrogen Codoped Carbon Nanospheres as Efficient Polysulfide Mediator for High-Performance Lithium-Sulfur Batteries.

Wang Jin J   Yang Hao H   Chen Zhen Z   Zhang Lili L   Liu Jilei J   Liang Pei P   Yang Hui H   Shen Xiaodong X   Shen Ze Xiang ZX  

Advanced science (Weinheim, Baden-Wurttemberg, Germany) 20180908 11

Lithium-sulfur batteries are regarded as very promising energy storage devices due to their high energy density, low cost, and environmental friendliness; however, their insulating properties and the instability of sulfur-based electrodes impede the practical applications of Li-S batteries. Here, a versatile strategy to synthesize double-shelled nitrogen and phosphorus codoped carbon spheres (NPDSCS) as an efficient sulfur host for Li-S batteries is reported. With strong trapping, good affinity,  ...[more]

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