Dataset Information

A Call for an Aloft Air Quality Monitoring Network: Need, Feasibility, and Potential Value.

ABSTRACT: Changing precursor emission patterns in conjunction with stringent health protective air quality standards necessitate accurate quantification of nonlocal contributions to ozone pollution at a location due to atmospheric transport, that by nature predominantly occurs aloft nocturnally. Concerted efforts to characterize ozone aloft on a continuous basis to quantify its contribution to ground-level concentrations, however, are lacking. By applying our classical understanding of air pollution dynamics to analyze variations in widespread surface-level ozone measurements, in conjunction with process-based interpretation from a comprehensive air pollution modeling system and detailed backward-sensitivity calculations that quantitatively link surface-level and aloft pollution, we show that accurate quantification of the amount of ozone in the air entrained from aloft every morning as the atmospheric boundary layer grows is the key missing component for characterizing background pollution at a location, and we propose a cost-effective continuous aloft ozone measurement strategy to address critical scientific gaps in current air quality management. Continuous aloft air pollution measurements can be achieved cost-effectively through leveraging advances in sensor technology and proliferation of tall telecommunications masts. Resultant improvements in ozone distribution characterization at 400-500 m altitude are estimated to be 3-4 times more effective in characterizing the surface-level daily maximum 8-h average ozone (DM8O3) than improvements from surface measurements since they directly quantify the amount of pollution imported to a location and furnish key missing information on processes and sources regulating background ozone and its modulation of ground-level concentrations. Since >80% of the DM8O3 sensitivity to tropospheric ozone is potentially captured through measurements between 200 and 1200 m altitude (a possible design goal for future remote sensing instrumentation), their assimilation will dramatically improve air quality forecast and health advisories.

SUBMITTER: Mathur R

PROVIDER: S-EPMC6261453 | biostudies-literature | 2018 Oct

REPOSITORIES: biostudies-literature

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A Call for an Aloft Air Quality Monitoring Network: Need, Feasibility, and Potential Value.

Mathur Rohit R Hogrefe Christian C Hakami Amir A Zhao Shunliu S Szykman James J Hagler Gayle G

Environmental science & technology 20180918 19

Changing precursor emission patterns in conjunction with stringent health protective air quality standards necessitate accurate quantification of nonlocal contributions to ozone pollution at a location due to atmospheric transport, that by nature predominantly occurs aloft nocturnally. Concerted efforts to characterize ozone aloft on a continuous basis to quantify its contribution to ground-level concentrations, however, are lacking. By applying our classical understanding of air pollution dynam ...[more]

PMID: 30180558

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Project description:Analyses of the relationships between climate, air substances and health usually concentrate on urban environments because of increased urban temperatures, high levels of air pollution and the exposure of a large number of people compared to rural environments. Ongoing urbanization, demographic ageing and climate change lead to an increased vulnerability with respect to climate-related extremes and air pollution. However, systematic analyses of the specific local-scale characteristics of health-relevant atmospheric conditions and compositions in urban environments are still scarce because of the lack of high-resolution monitoring networks. In recent years, low-cost sensors (LCS) became available, which potentially provide the opportunity to monitor atmospheric conditions with a high spatial resolution and which allow monitoring directly at vulnerable people. In this study, we present the atmospheric exposure low-cost monitoring (AELCM) system for several air substances like ozone, nitrogen dioxide, carbon monoxide and particulate matter, as well as meteorological variables developed by our research group. The measurement equipment is calibrated using multiple linear regression and extensively tested based on a field evaluation approach at an urban background site using the high-quality measurement unit, the atmospheric exposure monitoring station (AEMS) for meteorology and air substances, of our research group. The field evaluation took place over a time span of 4 to 8 months. The electrochemical ozone sensors (SPEC DGS-O3: R2: 0.71-0.95, RMSE: 3.31-7.79 ppb) and particulate matter sensors (SPS30 PM1/PM2.5: R2: 0.96-0.97/0.90-0.94, RMSE: 0.77-1.07 µg/m3/1.27-1.96 µg/m3) showed the best performances at the urban background site, while the other sensors underperformed tremendously (SPEC DGS-NO2, SPEC DGS-CO, MQ131, MiCS-2714 and MiCS-4514). The results of our study show that meaningful local-scale measurements are possible with the former sensors deployed in an AELCM unit.

Dataset Information

A Call for an Aloft Air Quality Monitoring Network: Need, Feasibility, and Potential Value.

Publications

A Call for an Aloft Air Quality Monitoring Network: Need, Feasibility, and Potential Value.

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