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The use of columns of the zeolite clinoptilolite in the remediation of aqueous nuclear waste streams.


ABSTRACT: Mud Hills clinoptilolite has been used in an effluent treatment plant (SIXEP) at the Sellafield nuclear reprocessing site. This material has been used to remove 134/137Cs and 90Sr successfully from effluents for 3 decades. Samples of the zeolite have been tested in column experiments to determine their ability to remove radioactive Cs+ and Sr2+ ions under increasing concentrations of competing ions, Ca2+, Mg2+, Na+ and K+. These ions caused increased elution of Cs+ and Sr2+. Ca2+, Mg2+ and K+ were more effective competitors than Na+. For Na+, it was found that if concentration was reduced, then column performance recovered rapidly.

SUBMITTER: Dyer A 

PROVIDER: S-EPMC6267155 | biostudies-literature | 2018

REPOSITORIES: biostudies-literature

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The use of columns of the zeolite clinoptilolite in the remediation of aqueous nuclear waste streams.

Dyer Alan A   Hriljac Joe J   Evans Nick N   Stokes Ian I   Rand Peter P   Kellet Simon S   Harjula Risto R   Moller Teresia T   Maher Zoe Z   Heatlie-Branson Ross R   Austin Jonathan J   Williamson-Owens Scott S   Higgins-Bos Manon M   Smith Kurt K   O'Brien Luke L   Smith Nick N   Bryan Nick N  

Journal of radioanalytical and nuclear chemistry 20181122 3


Mud Hills clinoptilolite has been used in an effluent treatment plant (SIXEP) at the Sellafield nuclear reprocessing site. This material has been used to remove <sup>134/137</sup>Cs and <sup>90</sup>Sr successfully from effluents for 3 decades. Samples of the zeolite have been tested in column experiments to determine their ability to remove radioactive Cs<sup>+</sup> and Sr<sup>2+</sup> ions under increasing concentrations of competing ions, Ca<sup>2+</sup>, Mg<sup>2+</sup>, Na<sup>+</sup> and  ...[more]

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