Ontology highlight
ABSTRACT:
SUBMITTER: Kunsel T
PROVIDER: S-EPMC6345114 | biostudies-literature | 2019 Jan
REPOSITORIES: biostudies-literature
The journal of physical chemistry. B 20190103 2
We present a theory for modeling fluorescence-detected two-dimensional electronic spectroscopy of multichromophoric systems. The theory is tested by comparison of the predicted spectra of the light-harvesting complex LH2 with experimental data. A qualitative explanation of the strong cross-peaks as compared to conventional two-dimensional electronic spectra is given. The strong cross-peaks are attributed to the clean ground-state signal that is revealed when the annihilation of exciton pairs cre ...[more]