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Radiation tolerance of two-dimensional material-based devices for space applications.


ABSTRACT: Characteristic for devices based on two-dimensional materials are their low size, weight and power requirements. This makes them advantageous for use in space instrumentation, including photovoltaics, batteries, electronics, sensors and light sources for long-distance quantum communication. Here we present a comprehensive study on combined radiation effects in Earth's atmosphere on various devices based on these nanomaterials. Using theoretical modeling packages, we estimate relevant radiation levels and then expose field-effect transistors, single-photon sources and monolayers as building blocks for future electronics to ?-rays, protons and electrons. The devices show negligible change in performance after the irradiation, suggesting robust suitability for space use. Under excessive ?-radiation, however, monolayer WS2 shows decreased defect densities, identified by an increase in photoluminescence, carrier lifetime and a change in doping ratio proportional to the photon flux. The underlying mechanism is traced back to radiation-induced defect healing, wherein dissociated oxygen passivates sulfur vacancies.

SUBMITTER: Vogl T 

PROVIDER: S-EPMC6416293 | biostudies-literature | 2019 Mar

REPOSITORIES: biostudies-literature

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Radiation tolerance of two-dimensional material-based devices for space applications.

Vogl Tobias T   Sripathy Kabilan K   Sharma Ankur A   Reddy Prithvi P   Sullivan James J   Machacek Joshua R JR   Zhang Linglong L   Karouta Fouad F   Buchler Ben C BC   Doherty Marcus W MW   Lu Yuerui Y   Lam Ping Koy PK  

Nature communications 20190313 1


Characteristic for devices based on two-dimensional materials are their low size, weight and power requirements. This makes them advantageous for use in space instrumentation, including photovoltaics, batteries, electronics, sensors and light sources for long-distance quantum communication. Here we present a comprehensive study on combined radiation effects in Earth's atmosphere on various devices based on these nanomaterials. Using theoretical modeling packages, we estimate relevant radiation l  ...[more]

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