Dataset Information

Characterization and health risk assessment of PM_2.5-bound polycyclic aromatic hydrocarbons in 5 urban cities of Zhejiang Province, China.

ABSTRACT: In 2015, we measured polycyclic aromatic hydrocarbons (PAHs) in atmospheric fine particulate matter (PM_2.5) collected from 5 cities in Zhejiang Province. The mean toxic equivalent quotient (TEQ) values of benzo(a)pyrene (BaP) ranged between 1.2-3.1 ng/m³. The BaP-TEQ displayed seasonal trends, such that winter > spring and autumn > summer. During the winter, the most abundant individual PAHs were 4-6ring PAHs (84.04-91.65%). The median daily intake of atmospheric PAHs ranged between 2.0-7.4 ng/day for all populations, with seasonal trends identical to that of BaP-TEQ. The 95^th incremental lifetime cancer risk (ILCR) values induced by PM_2.5-bound PAHs were far lower than 10^-6 for all populations. The data suggested that the pollution levels in the 5 Zhejiang Province cities were higher than the Chinese National Ambient Air Quality Standard (NAAQS). In the future, relevant measures should be taken to control atmospheric PAHs, especially 4-6 ring PAHs. The data also revealed no obvious cancer risk for populations residing in these 5 cities of Zhejiang Province.

SUBMITTER: Mo Z

PROVIDER: S-EPMC6513845 | biostudies-literature | 2019 May

REPOSITORIES: biostudies-literature

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Characterization and health risk assessment of PM2.5-bound polycyclic aromatic hydrocarbons in 5 urban cities of Zhejiang Province, China.

Mo Zhe Z Wang Zhifang Z Mao Guangming G Pan Xuejiao X Wu Lizhi L Xu Peiwei P Chen Shuchang S Wang Aihong A Zhang Yongli Y Luo Jinbin J Ye Xialiang X Wang Xiaofeng X Chen Zhijian Z Lou Xiaoming X

Scientific reports 20190513 1

In 2015, we measured polycyclic aromatic hydrocarbons (PAHs) in atmospheric fine particulate matter (PM2.5) collected from 5 cities in Zhejiang Province. The mean toxic equivalent quotient (TEQ) values of benzo(a)pyrene (BaP) ranged between 1.2-3.1 ng/m3. The BaP-TEQ displayed seasonal trends, such that winter > spring and autumn > summer. During the winter, the most abundant individual PAHs were 4-6ring PAHs (84.04-91.65%). The median daily intake of atmospheric PAHs range ...[more]

PMID: 31086237

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Project description:The Polycyclic Aromatic Hydrocarbons (PAHs) bound to ambient fine Particular Matter (PM2.5) are currently drawing a lot of attention due to their adverse health effects increasing lung cancer risk in humans. In this study, The PM2.5 samples were collected by high volume air samplers simultaneously from three different sites (high-traffic roadside, urban background, and remote suburban) in Tehran, Iran during warm and cold seasons (from July 2018 to March 2019), and 16 PAHs were analyzed using Gas Chromatography-Mass Spectrometry (GC-MS). Unlike previous studies, a remote suburban area was chosen so as to observe the spatial differentiation in PM2.5-bound PAH characteristics. In high-traffic roadside site, the average concentration of total PM2.5-bound PAHs (ƩPAHs) was 3.7 times the concentration value in remote suburban area. Average (ƩPAHs) ranged from 5.54 ng/m3 for remote suburban area to 20.67 ng/m3 for high-traffic roadside site. In all sites, seasonal trends of PAH concentrations elucidated high concentrations in the cold season and low concentrations in the warm season. Correlation analysis between ƩPAHs and atmospheric factors (meteorology parameters and criteria air pollutants) indicated the heterogeneous processes play an important role in the level of PAHs. The results of diagnostic ratio (DR) analysis disclosed that the dominant source of PM2.5-bound PAHs was the combustion of liquid fossil fuels. Despite the fact that incremental lifetime cancer risk (ILCR) via inhaling PM2.5-bound PAHs varied significantly in high-traffic roadside site and remote suburban site, its value was beyond the acceptable risk level in both sites. Our results suggested that effective regulations are needed to monitor PAHs concentrations and reduce PAHs emissions from liquid fossil fuel combustion so as to mitigate the potential carcinogenic risk of PAHs in ambient air.Supplementary informationThe online version contains supplementary material available at 10.1007/s40201-022-00821-2.

Project description:Electronic waste (e-waste) disposal and recycling activities such as burning and smelting can emit particulate matter (PM), polycyclic aromatic hydrocarbons (PAHs), and other pollutants that expose workers and nearby communities. At informal e-waste recycling facilities, both emission controls and protective measures for workers are absent. This study characterizes personal exposures (breathing zone) of PM and PAHs of e-waste workers at the large Agbogbloshie e-waste site in Accra, Ghana. We collected gravimetric and optical measurements of PM2.5 and PM10 using shift samples for workers and for an age- and gender-matched reference population. PM2.5 filters were analyzed for 26 PAHs using gas chromatography/mass spectroscopy. Among e-waste workers, PM2.5 and PM10 concentrations were 99 ± 56 and 218 ± 158 µg/m3 (median ± interquartile range, optical measurements), respectively; these levels were 78 and 57% higher, respectively, than levels measured at a fixed site that was centrally located at the waste site. In the reference community, breathing zone PM2.5 and PM10 levels were lower, 49 ± 20 and 131 ± 108 µg/m3, respectively, and the fraction of coarse PM was larger. We detected all 26 target PAHs, of which naphthalene and phenanthrene were the most abundant. PAH concentrations were weakly correlated to PM levels, but PAH abundances, representing the fraction of PAH mass to the total PM2.5 mass collected, were strongly and inversely correlated to PM levels, suggesting multiple and different sources of PAHs and PM that affected exposures. Both PM and PAH levels were elevated for workers performing burning and dismantling, and both exceeded standards or risk-based guidelines, e.g., lifetime excess cancer risks for several PAHs were in the 10-4 to 10-6 range, indicating the need to reduce emissions as well as provide respiratory protection. The study emphasizes the importance of using personal and shift samples to accurately characterize worker exposure.

Dataset Information

Characterization and health risk assessment of PM_2.5-bound polycyclic aromatic hydrocarbons in 5 urban cities of Zhejiang Province, China.

Publications

Characterization and health risk assessment of PM<sub>2.5</sub>-bound polycyclic aromatic hydrocarbons in 5 urban cities of Zhejiang Province, China.

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