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Li(Cd,Mn)P: a new cadmium based diluted ferromagnetic semiconductor with independent spin & charge doping.


ABSTRACT: We report a new diluted ferromagnetic semiconductor Li1+y(Cd,Mn)P, wherein carrier is doped via excess Li while spin is doped by isovalence substitution of Mn2+ into Cd2+. The extended Cd 4d-orbitals lead to more itinerant characters of Li1+y(Cd,Mn)P than that of analogous Li1+y(Zn,Mn)P. A higher Curie temperature of 45?K than that for Li1+y(Zn,Mn)P is obtained in Li1+y(Cd,Mn)P polycrystalline samples by Arrott plot technique. The p-type carriers are determined by Hall effect measurements. The first principle calculations and X-ray diffraction measurements indicate that occupation of excess Li is at Cd sites rather than the interstitial site. Consequently holes are doped by excess Li substitution. More interestingly Li1+y(Cd,Mn)P shows a very low coercive field (<100?Oe) and giant negative magnetoresistance (~80%) in ferromagnetic state that will benefit potential spintronics applications.

SUBMITTER: Han W 

PROVIDER: S-EPMC6522530 | biostudies-literature | 2019 May

REPOSITORIES: biostudies-literature

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Li(Cd,Mn)P: a new cadmium based diluted ferromagnetic semiconductor with independent spin & charge doping.

Han W W   Chen B J BJ   Gu B B   Zhao G Q GQ   Yu S S   Wang X C XC   Liu Q Q QQ   Deng Z Z   Li W M WM   Zhao J F JF   Cao L P LP   Peng Y Y   Shen X X   Zhu X H XH   Yu R C RC   Maekawa S S   Uemura Y J YJ   Jin C Q CQ  

Scientific reports 20190516 1


We report a new diluted ferromagnetic semiconductor Li<sub>1+y</sub>(Cd,Mn)P, wherein carrier is doped via excess Li while spin is doped by isovalence substitution of Mn<sup>2+</sup> into Cd<sup>2+</sup>. The extended Cd 4d-orbitals lead to more itinerant characters of Li<sub>1+y</sub>(Cd,Mn)P than that of analogous Li<sub>1+y</sub>(Zn,Mn)P. A higher Curie temperature of 45 K than that for Li<sub>1+y</sub>(Zn,Mn)P is obtained in Li<sub>1+y</sub>(Cd,Mn)P polycrystalline samples by Arrott plot tec  ...[more]

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