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Experimental study on removing heavy metals from the municipal solid waste incineration fly ash with the modified electrokinetic remediation device.

ABSTRACT: The MSWI fly ash which contains a large number of heavy metal substances is a subsidiary product of waste incineration power generation technology. If the MSWI fly ash is disposed improperly, heavy metal pollutants will pose a great threat to environmental safety and human health. Based on the technology of electrokinetic remediation, the feasibility of removing heavy metal pollutants from the MSWI fly ash using a modified electrokinetic remediation device - cylinder device was evaluated in this study. Differing from the traditional cuboid device with the volume ratio of the cathode chamber to the anode chamber being 1:1, the volume ratio of the cathode chamber to the anode chamber of the cylinder device was 16:1. Changes in parameters, such as pH values and conductivity in the cathode and the anode chambers as well as current and voltage in the sample area were analysed under the voltage gradient of 2?V/cm. After the experiment, the average removal efficiencies for Zn, Pb, Cd and Cu in the sample area were 53.2%, 31.4%, 42.3% and 30.7%, respectively. It indicates that the cylinder device is effective in removing heavy metals from the MSWI fly ash. Adopting the cylinder device for the experimental study on the electrokinetic remediation technology could provide a better way of thinking for the future engineering practices and applications.

SUBMITTER: Ji H

PROVIDER: S-EPMC6547674 | biostudies-literature | 2019 Jun

REPOSITORIES: biostudies-literature

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Experimental study on removing heavy metals from the municipal solid waste incineration fly ash with the modified electrokinetic remediation device.

Ji Hong H Huang Weiqiu W Xing Zhixiang Z Zuo Jiaqi J Wang Zhuang Z Yang Ke K

Scientific reports 20190604 1

The MSWI fly ash which contains a large number of heavy metal substances is a subsidiary product of waste incineration power generation technology. If the MSWI fly ash is disposed improperly, heavy metal pollutants will pose a great threat to environmental safety and human health. Based on the technology of electrokinetic remediation, the feasibility of removing heavy metal pollutants from the MSWI fly ash using a modified electrokinetic remediation device - cylinder device was evaluated in this ...[more]

PMID: 31164661

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Project description:Incineration has emerged as one of the acceptable ways to treat municipal solid waste (MSW) due to its potential in reducing the mass and volume of the waste. However, it produces two major by-product residues, namely MSW-bottom ash (MSW-BA) and MSW-fly ash (MSW-FA). These residues have gained great attention to their hazardous nature and potential to be reused and recycled. In this paper, the physicochemical characterizations of the MSW-BA and the MSW-FA were performed, followed by a systematic investigation of metals extraction from MSW-BA and MSW-FA. Various extracting agents were used to investigate the possibility to extract 21 metals including cadmium (Cd), vanadium (V), chromium (Cr), and lead (Pb). It was revealed that some metals were present in a high amount in the MSW-BA while other metals were higher in the MSW-FA. Moreover, the energy-dispersive X-ray spectroscopy results revealed that the MSW-BA was dominated by oxygen (O) 55.4 ±0.6 wt%, silicon (Si) 22.5 ±0.3 wt%, and calcium (Ca) 18.5 ±0.2 wt%. On the other hand, the MSW-FA was enriched with Ca 45.2 ±0.5 wt%, and O 40.3 ±0.4 wt%. From the scanning electron microscopy, the MSW-BA was observed as flaky with an irregular surface that consisted of large pores, while, the MSW-FA was present as agglomerated particles and had a bimodal distribution. Moreover, Fourier transform infrared spectroscopy revealed that Al-Fe-OH, Al-Al-OH, Si-O, C-O, and C-H were some of the major functional groups present in the ashes. The F-tests concluded that the metal extraction from the MSW-BA and MSW-FA were significantly affected by the acid type. it is concluded that nitric acid and phosphoric acid were the best-suited acid for the MSW-BA while sulfuric acid and phosphoric acid for the MSW-FA. More than 11 wt% of Cd and 9 wt% of Cu were extracted from MSW-BA while 6 wt% of Pb and 4.5 wt% of V were extracted from the MSW-FA. The present methodology is an interesting development in metal extraction from the MSW-BA and the MSW-FA, which can develop in a cost-effective and sustainable option to utilize MSW.

Dataset Information

Experimental study on removing heavy metals from the municipal solid waste incineration fly ash with the modified electrokinetic remediation device.

Publications

Experimental study on removing heavy metals from the municipal solid waste incineration fly ash with the modified electrokinetic remediation device.

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