Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La_2-x Ba _x CuO₄.

ABSTRACT: Charge order is universal among high-T _c cuprates, but its relation to superconductivity is unclear. While static order competes with superconductivity, dynamic order may be favorable and even contribute to Cooper pairing. Using time-resolved resonant soft x-ray scattering at a free-electron laser, we show that the charge order in prototypical La_2-x Ba _x CuO₄ exhibits transverse fluctuations at picosecond time scales. These sub-millielectron volt excitations propagate by Brownian-like diffusion and have an energy scale remarkably close to the superconducting T _c. At sub-millielectron volt energy scales, the dynamics are governed by universal scaling laws defined by the propagation of topological defects. Our results show that charge order in La_2-x Ba _x CuO₄ exhibits dynamics favorable to the in-plane superconducting tunneling and establish time-resolved x-rays as a means to study excitations at energy scales inaccessible to conventional scattering techniques.

SUBMITTER: Mitrano M 

PROVIDER: S-EPMC6697434 | biostudies-literature | 2019 Aug

REPOSITORIES: biostudies-literature