Dataset Information

A global view on the effect of water uptake on aerosol particle light scattering.

ABSTRACT: A reference dataset of multi-wavelength particle light scattering and hemispheric backscattering coefficients for different relative humidities (RH) between RH?=?30 and 95% and wavelengths between ??=?450?nm and 700?nm is described in this work. Tandem-humidified nephelometer measurements from 26 ground-based sites around the globe, covering multiple aerosol types, have been re-analysed and harmonized into a single dataset. The dataset includes multi-annual measurements from long-term monitoring sites as well as short-term field campaign data. The result is a unique collection of RH-dependent aerosol light scattering properties, presented as a function of size cut. This dataset is important for climate and atmospheric model-measurement inter-comparisons, as a means to improve model performance, and may be useful for satellite and remote sensing evaluation using surface-based, in-situ measurements.

SUBMITTER: Burgos MA

PROVIDER: S-EPMC6706437 | biostudies-literature | 2019 Aug

REPOSITORIES: biostudies-literature

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A global view on the effect of water uptake on aerosol particle light scattering.

Burgos María A MA Andrews Elisabeth E Titos Gloria G Alados-Arboledas Lucas L Baltensperger Urs U Day Derek D Jefferson Anne A Kalivitis Nikos N Mihalopoulos Nikos N Sherman James J Sun Junying J Weingartner Ernest E Zieger Paul P

Scientific data 20190822 1

A reference dataset of multi-wavelength particle light scattering and hemispheric backscattering coefficients for different relative humidities (RH) between RH = 30 and 95% and wavelengths between λ = 450 nm and 700 nm is described in this work. Tandem-humidified nephelometer measurements from 26 ground-based sites around the globe, covering multiple aerosol types, have been re-analysed and harmonized into a single dataset. The dataset includes multi-annual measurements from long-term monitoring ...[more]

PMID: 31439840

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Project description:The aerosol scattering coefficient and Ångström exponent (AE) are important parameters in the understanding of aerosol optical properties and aerosol direct effect. These parameters are usually measured by a nephelometer network which is under-represented geographically; however, a rapid growth of air-pollution monitoring, using low-cost particle sensors, may extend observation networks. This paper presents the results of co-located measurements of aerosol optical properties, such as the aerosol scattering coefficient and the scattering AE, using low-cost sensors and using a scientific-grade polar Aurora 4000 nephelometer. A high Pearson correlation coefficient (0.94-0.96) between the low-cost particulate matter (PM) mass concentration and the aerosol scattering coefficient was found. For the PM10 mass concentration, the aerosol scattering coefficient relation is linear for the Dfrobot SEN0177 sensor and non-linear for the Alphasense OPC-N2 device. After regression analyses, both low-cost instruments provided the aerosol scattering coefficient with a similar mean square error difference (RMSE) of about 20 Mm-1, which corresponds to about 27% of the mean aerosol scattering coefficient. The relative uncertainty is independent of the pollution level. In addition, the ratio of aerosol number concentration between different bins showed a significant statistical (95% of confidence level) correlation with the scattering AE. For the SEN0177, the ratio of the particle number in bin 1 (radius of 0.15-0.25 µm) to bin 4 (radius of 1.25-2.5 µm) was a linear function of the scattering AE, with a Pearson correlation coefficient of 0.74. In the case of OPC-N2, the best correlation (r = 0.66) was found for the ratio between bin 1 (radius of 0.19-0.27 µm) and bin 2 (radius of 0.27-0.39 µm). Comparisons of an estimated scattering AE from a low-cost sensor with Aurora 4000 are given with the RMSE of 0.23-0.24, which corresponds to 16-19%. In addition, a three-year (2016-2019) observation by SEN0177 indicates that this sensor can be used to determine an annual cycle as well as a short-term variability.

Dataset Information

A global view on the effect of water uptake on aerosol particle light scattering.

Publications

A global view on the effect of water uptake on aerosol particle light scattering.

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