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Sn-Based Perovskite for Highly Sensitive Photodetectors.


ABSTRACT: Organic-inorganic hybrid perovskites have emerged as promising functional materials for high-performance photodetectors. However, the toxicity of Pb and the lack of internal gain mechanism in typical perovskites significantly hinder their practical applications. Herein, a low-voltage and high-performance photodetector based on a single layer of lead-free Sn-based perovskite film is reported. The device shows broadband response from ultraviolet to near-infrared light with a responsivity up to 105 A W-1 and a high gain at a low operating voltage. The outstanding performance is attributed to the high hole mobility, p-doping nature, and excellent optoelectronic properties of the Sn-based perovskite. Moreover, the device is assembled on a flexible substrate and demonstrates both high sensitivity and good bending stability. This work demonstrates a route for realizing nontoxic, low-cost, and high-performance perovskite photodetectors with a simple device structure.

SUBMITTER: Liu CK 

PROVIDER: S-EPMC6724360 | biostudies-literature | 2019 Sep

REPOSITORIES: biostudies-literature

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Sn-Based Perovskite for Highly Sensitive Photodetectors.

Liu Chun-Ki CK   Tai Qidong Q   Wang Naixiang N   Tang Guanqi G   Loi Hok-Leung HL   Yan Feng F  

Advanced science (Weinheim, Baden-Wurttemberg, Germany) 20190713 17


Organic-inorganic hybrid perovskites have emerged as promising functional materials for high-performance photodetectors. However, the toxicity of Pb and the lack of internal gain mechanism in typical perovskites significantly hinder their practical applications. Herein, a low-voltage and high-performance photodetector based on a single layer of lead-free Sn-based perovskite film is reported. The device shows broadband response from ultraviolet to near-infrared light with a responsivity up to 10<  ...[more]

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