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Combined Use of Anisotropic Silver Nanoprisms with Different Aspect Ratios for Multi-Mode Plasmon-Exciton Coupling.


ABSTRACT: Absorption enhancement based on interaction between the localized surface plasmon (LSP) and molecular exciton is one of the most important phenomena for the development of high-performance solar devices. In this study, hybrids of plasmonic metal nanoparticles and dye molecules have been developed, which exhibit enhanced absorption at precisely tuned wavelengths in a visible region. The hybrids consist of a porphyrin derivative, which has four absorption peaks (Q-bands) in a range of 500-700 nm, and triangular silver nanoprisms (AgPRs), which are developed by us to exhibit precisely tuned LSP resonance wavelengths. Absorption enhancement over the whole Q-band range is induced by the combined use of three kinds of AgPRs of different aspect ratios. Furthermore, the quantitative evaluation of absorption enhancement based on the LSP-based fluorescence enhancement phenomenon has demonstrated that efficient absorption enhancement can be effected at multiple wavelengths.

SUBMITTER: Takeshima N 

PROVIDER: S-EPMC6965570 | biostudies-literature | 2020 Jan

REPOSITORIES: biostudies-literature

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Combined Use of Anisotropic Silver Nanoprisms with Different Aspect Ratios for Multi-Mode Plasmon-Exciton Coupling.

Takeshima Naoto N   Sugawa Kosuke K   Tahara Hironobu H   Jin Shota S   Noguchi Masaki M   Hayakawa Yutaro Y   Yamakawa Yuhei Y   Otsuki Joe J  

Nanoscale research letters 20200116 1


Absorption enhancement based on interaction between the localized surface plasmon (LSP) and molecular exciton is one of the most important phenomena for the development of high-performance solar devices. In this study, hybrids of plasmonic metal nanoparticles and dye molecules have been developed, which exhibit enhanced absorption at precisely tuned wavelengths in a visible region. The hybrids consist of a porphyrin derivative, which has four absorption peaks (Q-bands) in a range of 500-700 nm,  ...[more]

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