Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations.
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ABSTRACT:
SUBMITTER: Liu L
PROVIDER: S-EPMC7042275 | biostudies-literature | 2020 Feb
REPOSITORIES: biostudies-literature
Publications
Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations.
Liu Lili L Nakouzi Elias E Sushko Maria L ML Schenter Gregory K GK Mundy Christopher J CJ Chun Jaehun J De Yoreo James J JJ
Nature communications 20200225 1
The interplay between crystal and solvent structure, interparticle forces and ensemble particle response dynamics governs the process of crystallization by oriented attachment (OA), yet a quantitative understanding is lacking. Using ZnO as a model system, we combine in situ TEM observations of single particle and ensemble assembly dynamics with simulations of interparticle forces and responses to relate experimentally derived interparticle potentials to the underlying interactions. We show that ...[more]
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