Dynamic inferential NO x emission prediction model with delay estimation for SCR de-NO x process in coal-fired power plants.
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ABSTRACT:
SUBMITTER: Yan L
PROVIDER: S-EPMC7062099 | biostudies-literature |
REPOSITORIES: biostudies-literature
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Project description:AbstractCoal is expected to remain a significant power supply source worldwide and shifting to carbon-neutral fuels will be challenging because of growing electricity demand and booming industrialization. At the same time, coal consumption results in severe air pollution and health concerns. Improvement in emission control technologies is a key to improving air quality in coal power plants. Many scientists reported removing air pollutants individually via conventional control methods. However, controlling multiple pollutants combinedly using the latest techniques is rarely examined. Therefore, this paper overviews the current and advanced physical technologies to control multi-air pollutants synergistically, including carbon control technologies. Also, the paper aims to examine how potential air pollutants (e.g., PM2.5, SO2, NOx, CO2), including mercury from the coal-fired power plants, cause environmental impacts. The data synthesis shows that coal quality is the most significant factor for increasing air emissions, regardless of power plant capacity. It is found that selecting techniques is critical for new and retrofitted plants depending on the aging of a power plant and other socio-economic factors. Considering the future perspective, this paper discusses possible pathways to transform from linear to a circular economy in a coal power plant sector, such as utilizing energy losses through energy-efficient processes and reuse of syngas. The article provides an in-depth analysis of advanced cost-effective techniques that would help to control the air pollution level. Additionally, a life cycle assessment-based decision-making framework is proposed that would assist the stakeholders in achieving net-zero emissions and offset the financial burden for air pollution control in coal-fired power plants.Graphical abstractSupplementary informationThe online version contains supplementary material available at 10.1007/s10098-022-02328-8.
| S-EPMC9075710 | biostudies-literature
Project description:BackgroundCoal-fired power plants are a major source of air pollution that can impact children's health. Limited research has explored if proximity to coal-fired power plants contributes to children's neurobehavioral disorders.ObjectiveThis community-based study collected primary data to investigate the relationships of residential proximity to power plants and neurobehavioral problems in children.Methods235 participants aged 6-14 years who lived within 10 miles of two power plants were recruited. Exposure to particulate matter ≤10 μm (PM10) was measured in children's homes using personal modular impactors. Neurobehavioral symptoms were assessed using the Child Behavior Checklist (CBCL). Multiple regression models were performed to test the hypothesized associations between proximity/exposure and neurobehavioral symptoms. Geospatial statistical methods were used to map the spatial patterns of exposure and neurobehavioral symptoms.ResultsA small proportion of the variations of neurobehavioral problems (social problems, affective problems, and anxiety problems) were explained by the regression models in which distance to power plants, traffic proximity, and neighborhood poverty was statistically associated with the neurobehavioral health outcomes. Statistically significant hot spots of participants who had elevated levels of attention deficit hyperactivity disorder, anxiety, and social problems were observed in the vicinity of the two power plants.SignificanceResults of this study suggest an adverse impact of proximity to power plants on children's neurobehavioral health. Although coal-fired power plants are being phased out in the US, health concern about exposure from coal ash storage facilities remains. Furthermore, other countries in the world are increasing coal use and generating millions of tons of pollutants and coal ash. Findings from this study can inform public health policies to reduce children's risk of neurobehavioral symptoms in relation to proximity to power plants.
| S-EPMC8275639 | biostudies-literature
Project description:BACKGROUND:Exposure to ambient particulate matter generated from coal-fired power plants induces long-term health consequences. However, epidemiologic studies have not yet focused on attributing these health burdens specifically to energy consumption, impeding targeted intervention policies. We hypothesize that the generating capacity of coal-fired power plants may be associated with lung cancer incidence at the national level. METHODS:Age- and sex-adjusted lung cancer incidence from every country with electrical plants using coal as primary energy supply were followed from 2000 to 2016. We applied a Poisson regression longitudinal model, fitted using generalized estimating equations, to estimate the association between lung cancer incidence and per capita coal capacity, adjusting for various behavioral and demographic determinants and lag periods. RESULTS:The average coal capacity increased by 1.43 times from 16.01 gigawatts (GW) (2000~2004) to 22.82 GW (2010~2016). With 1?kW (KW) increase of coal capacity per person in a country, the relative risk of lung cancer increases by a factor of 59% (95% CI?=?7.0%~?135%) among males and 85% (95% CI?=?22%~?182%) among females. Based on the model, we estimate a total of 1.37 (range?=?1.34 ~?1.40) million standardized incident cases from lung cancer will be associated with coal-fired power plants in 2025. CONCLUSIONS:These analyses suggest an association between lung cancer incidence and increased reliance on coal for energy generation. Such data may be helpful in addressing a key policy question about the externality costs and estimates of the global disease burden from preventable lung cancer attributable to coal-fired power plants at the national level.
| S-EPMC6350330 | biostudies-literature
Project description:We examine the health implications of electricity generation from the 2018 stock of coal-fired power plants in India, as well as the health impacts of the expansion in coal-fired generation capacity expected to occur by 2030. We estimate emissions of SO2, NOX, and particulate matter 2.5 μm (PM2.5) for each plant and use a chemical transport model to estimate the impact of power plant emissions on ambient PM2.5 Concentration-response functions from the 2019 Global Burden of Disease (GBD) are used to project the impacts of changes in PM2.5 on mortality. Current plus planned plants will contribute, on average, 13% of ambient PM2.5 in India. This reflects large absolute contributions to PM2.5 in central India and parts of the Indo-Gangetic plain (up to 20 μg/m3). In the south of India, coal-fired power plants account for 20-25% of ambient PM2.5 We estimate 112,000 deaths are attributable annually to current plus planned coal-fired power plants. Not building planned plants would avoid at least 844,000 premature deaths over the life of these plants. Imposing a tax on electricity that reflects these local health benefits would incentivize the adoption of renewable energy.
| S-EPMC7865184 | biostudies-literature
Project description:Mercury contamination in food can pose serious health risks to consumers and coal-fired power plants have been identified as the major source of mercury emissions. To assess the current state of mercury pollution in food crops grown near coal-fired power plants, we measured the total mercury concentration in vegetables and grain crops collected from farms located near two coal-fired power plants. We found that 79% of vegetable samples and 67% of grain samples exceeded the PTWI's food safety standards. The mercury concentrations of soil samples were negatively correlated with distances from the studied coal-fired power plants, and the mercury contents in lettuce, amaranth, water spinach, cowpea and rice samples were correlated with the mercury contents in soil samples, respectively. Also, the mercury concentrations in vegetable leaves were much higher than those in roots and the mercury content of vegetable leaves decreased significantly after water rinses. Our calculation suggests that probable weekly intake of mercury for local residents, assuming all of their vegetables and grains are from their own farmland, may exceed the toxicologically tolerable values allowed, and therefore long-term consumptions of these contaminated vegetables and grains may pose serious health risks.
| S-EPMC5422849 | biostudies-literature
Project description:Sulfur oxides (SOx), particularly SO2 emitted by coal-fired power plants, produce long-term risks for cardiovascular disease (CVD). We estimated the relative risks of CVD and ischemic heart disease (IHD) attributable to SOx emission globally. National SOx reduction achieved by emissions control systems was defined as the average SOx reduction percentage weighted by generating capacities of individual plants in a country. We analyzed the relative risk of CVD incidence associated with national SOx reduction for 13,581 coal-fired power-generating units in 79 countries. A 10% decrease in SOx emission was associated with 0.28% (males; 95%CI?=?-0.39%~0.95%) and 1.69% (females; 95%CI?=?0.99%~2.38%) lower CVD risk. The effects on IHD were?>?2 times stronger among males than females (2.78%, 95%CI?=?1.99%~3.57% vs. 1.18%, 95%CI?=?0.19%~2.17%). Further, 1.43% (males) and 8.00% (females) of CVD cases were attributable to suboptimal SOx reduction. Thus, enhancing regulations on SOx emission control represents a target for national and international intervention to prevent CVD.
| S-EPMC5805744 | biostudies-literature
Project description:Climate policies that achieve air quality co-benefits can better align developing countries' national interests with global climate mitigation. Since the effects of air pollutants are highly dependent on source locations, spatially nuanced policies are crucial to maximizing the achievement of co-benefits. Using the coal power industry as a case study, this study presents an interdisciplinary approach to assessing facility level co-benefits at every specific source location in China. We find that co-benefits range from US$51-$278 per ton CO2 reduction nationwide and are highly heterogeneous spatially, with "hotspot" regions that should be the priority of emissions reduction policies, and that provinces should use different techno-economic strategies to reduce emissions. The location-specific co-benefit value plus a carbon price serves as a unified environmental indicator that enables policy makers to more accurately understand the social costs of electricity generation from coal burning and provides a scientific framework for geographically nuanced policymaking.
| S-EPMC8629986 | biostudies-literature
Project description:We present airborne observations of gaseous reactive halogen species (HCl, Cl2, ClNO2, Br2,BrNO2, and BrCl), sulfur dioxide (SO2), and nonrefractory fine particulate chloride (pCl) and sulfate(pSO4) in power plant exhaust. Measurements were conducted during the Wintertime INvestigation of Transport, Emissions, and Reactivity campaign in February-March of 2015 aboard the NCAR-NSF C-130 aircraft. Fifty air mass encounters were identified in which SO2 levels were elevated ~5 ppb above ambient background levels and in proximity to operational power plants. Each encounter was attributed to one or more potential emission sources using a simple wind trajectory analysis. In case studies, we compare measured emission ratios to those reported in the 2011 National Emissions Inventory and present evidence of the conversion of HCl emitted from power plants to ClNO2. Taking into account possible chemical conversion downwind, there was general agreement between the observed and reported HCl: SO2 emission ratios. Reactive bromine species (Br2, BrNO2, and/or BrCl) were detected in the exhaust of some coal-fired power plants, likely related to the absence of wet flue gas desulfurization emission control technology. Levels of bromine species enhanced in some encounters exceeded those expected assuming all of the native bromide in coal was released to the atmosphere, though there was no reported use of bromide salts (as a way to reduce mercury emissions) during Wintertime INvestigation of Transport, Emissions, and Reactivity observations. These measurements represent the first ever in-flight observations of reactive gaseous chlorine and bromine containing compounds present in coal-fired power plant exhaust.
| S-EPMC6463521 | biostudies-literature
Project description:China's efforts to mitigate air pollution from its large-scale coal-fired power plants (CFPPs) have involved the widespread use of air pollution control devices (APCDs). However, the operation of these devices relies on substantial electricity generated by CFPPs, resulting in indirect CO2 emissions. The extent of CO2 emissions caused by APCDs in China remains uncertain. Here, using a plant-level dataset, we quantified the CO2 emissions associated with electricity consumption by APCDs in China's CFPPs. Our findings reveal a significant rise in CO2 emissions attributed to APCDs, increasing from 1.48 Mt in 2000 to 51.7 Mt in 2020. Moreover, the contribution of APCDs to total CO2 emissions from coal-fired power generation escalated from 0.12% to 1.19%. Among the APCDs, desulfurization devices accounted for approximately 80% of the CO2 emissions, followed by dust removal and denitration devices. Scenario analysis indicates that the lifespan of CFPPs will profoundly impact future emissions, with Nei Mongol, Shanxi, and Shandong provinces projected to exhibit the highest emissions. Our study emphasizes the urgent need for a comprehensive assessment of environmental policies and provides valuable insights for the integrated management of air pollutants and carbon emissions in CFPPs.
| S-EPMC10388163 | biostudies-literature
Project description:Hazardous heavy metal-laden coal combustion byproducts exposed to precipitation or surface/groundwater are of environmental concern. This study analyzed fly ash (FA) and desulfurization gypsum (FGD gypsum) samples obtained from 16 coal-fired power plants in Guizhou Province, China. A combination of field and laboratory studies was used to investigate the binding forms of lead (Pb), cadmium (Cd), and chromium (Cr) and their leaching characteristics under natural storage conditions. The results showed that there were significant proportions of residual states of these elements in FA (84-99% for Pb, 83-91% for Cd, and 73-97% for Cr), indicating a lack of migration to other environmental media. FGD gypsum contained high proportions of metals in migratable states, but the environmental risks were low due to their very low concentrations. The release of Pb, Cd, and Cr from FA and FGD gypsum into extracts varied according to pH. This is related to the form of each element in the solid and the series of reactions that occurs during the leaching process. However, aside from Cr in FA, all heavy metals in FA and FGD gypsum samples were present in concentrations below the relevant standards for landfill leachate, indicating very low release rates. The Cr levels (206-273 μg/L) in some of the FA extracts were higher than the limits for water pollution from domestic landfill, indicating that Cr in FA poses a leaching risk. The results of field leachate sampling and indoor simulated rainfall experiments further validated these findings, indicating that the release of Cr from stockpiled coal FA is a cause for concern.
| S-EPMC9566641 | biostudies-literature