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Water purification ultrafiltration membranes using nanofibers from unbleached and bleached rice straw.

ABSTRACT: There has been an increasing interest in recent years in isolating cellulose nanofibers from unbleached cellulose pulps for economic, environmental, and functional reasons. In the current work, cellulose nanofibers isolated from high-lignin unbleached neutral sulfite pulp were compared to those isolated from bleached rice straw pulp in making thin-film ultrafiltration membranes by vacuum filtration on hardened filter paper. The prepared membranes were characterized in terms of their microscopic structure, hydrophilicity, pure water flux, protein fouling, and ability to remove lime nanoparticles and purify papermaking wastewater effluent. Using cellulose nanofibers isolated from unbleached pulp facilitated the formation of a thin-film membrane (with a shorter filtration time for thin-film formation) and resulted in higher water flux than that obtained using nanofibers isolated from bleached fibers, without sacrificing its ability to remove the different pollutants.

SUBMITTER: Hassan ML

PROVIDER: S-EPMC7347555 | biostudies-literature | 2020 Jul

REPOSITORIES: biostudies-literature

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Water purification ultrafiltration membranes using nanofibers from unbleached and bleached rice straw.

Hassan Mohammad L ML Fadel Shaimaa M SM Abouzeid Ragab E RE Abou Elseoud Wafaa S WS Hassan Enas A EA Berglund Linn L Oksman Kristiina K

Scientific reports 20200709 1

There has been an increasing interest in recent years in isolating cellulose nanofibers from unbleached cellulose pulps for economic, environmental, and functional reasons. In the current work, cellulose nanofibers isolated from high-lignin unbleached neutral sulfite pulp were compared to those isolated from bleached rice straw pulp in making thin-film ultrafiltration membranes by vacuum filtration on hardened filter paper. The prepared membranes were characterized in terms of their microscopic ...[more]

PMID: 32647119

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Project description:Many current treatments for the reclamation of contaminated water sources are chemical-intensive, energy-intensive, and/or require posttreatment due to unwanted by-product formation. We demonstrate that through the integration of nanostructured materials, enzymatic catalysis, and iron-catalyzed free radical reactions within pore-functionalized synthetic membrane platforms, we are able to conduct environmentally important oxidative reactions for toxic organic degradation and detoxification from water without the addition of expensive or harmful chemicals. In contrast to conventional, passive membrane technologies, our approach utilizes two independently controlled, nanostructured membranes in a stacked configuration for the generation of the necessary oxidants. These include biocatalytic and organic/inorganic (polymer/iron) nanocomposite membranes. The bioactive (top) membrane contains an electrostatically immobilized enzyme for the catalytic production of one of the main reactants, hydrogen peroxide (H(2)O(2)), from glucose. The bottom membrane contains either immobilized iron ions or ferrihydrite/iron oxide nanoparticles for the decomposition of hydrogen peroxide to form powerful free radical oxidants. By permeating (at low pressure) a solution containing a model organic contaminant, such as trichlorophenol, with glucose in oxygen-saturated water through the membrane stack, significant contaminant degradation was realized. To illustrate the effectiveness of this membrane platform in real-world applications, membrane-immobilized ferrihydrite/iron oxide nanoparticles were reacted with hydrogen peroxide to form free radicals for the degradation of a chlorinated organic contaminant in actual groundwater. Although we establish the development of these nanostructured materials for environmental applications, the practical and methodological advances demonstrated here permit the extension of their use to applications including disinfection and/or virus inactivation.

Dataset Information

Water purification ultrafiltration membranes using nanofibers from unbleached and bleached rice straw.

Publications

Water purification ultrafiltration membranes using nanofibers from unbleached and bleached rice straw.

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