Highly Stretchable, Elastic, and Sensitive MXene-Based Hydrogel for Flexible Strain and Pressure Sensors.

ABSTRACT: Electronic skin is driving the next generation of cutting-edge wearable electronic products due to its good wearability and high accuracy of information acquisition. However, it remains a challenge to fulfill the requirements on detecting full-range human activities with existing flexible strain sensors. Herein, highly stretchable, sensitive, and multifunctional flexible strain sensors based on MXene- (Ti3C2T x -) composited poly(vinyl alcohol)/polyvinyl pyrrolidone double-network hydrogels were prepared. The uniformly distributed hydrophilic MXene nanosheets formed a three-dimensional conductive network throughout the hydrogel, endowing the flexible sensor with high sensitivity. The strong interaction between the double-network hydrogel matrix and MXene greatly improved the mechanical properties of the hydrogels. The resulting nanocomposited hydrogels featured great tensile performance (2400%), toughness, and resilience. Particularly, the as-prepared flexible pressure sensor revealed ultrahigh sensitivity (10.75?kPa-1) with a wide response range (0-61.5?kPa), fast response (33.5?ms), and low limit of detection (0.87?Pa). Moreover, the hydrogel-based flexible sensors, with high sensitivity and durability, could be employed to monitor full-range human motions and assembled into some aligned devices for subtle pressure detection, providing enormous potential in facial expression and phonation recognition, handwriting verification, healthy diagnosis, and wearable electronics.

SUBMITTER: Lu Y 

PROVIDER: S-EPMC7376495 | biostudies-literature | 2020

REPOSITORIES: biostudies-literature