Excess-entropy scaling in supercooled binary mixtures.
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ABSTRACT:
SUBMITTER: Bell IH
PROVIDER: S-EPMC7453028 | biostudies-literature | 2020 Aug
REPOSITORIES: biostudies-literature
Publications
Excess-entropy scaling in supercooled binary mixtures.
Bell Ian H IH Dyre Jeppe C JC Ingebrigtsen Trond S TS
Nature communications 20200827 1
Transport coefficients, such as viscosity or diffusion coefficient, show significant dependence on density or temperature near the glass transition. Although several theories have been proposed for explaining this dynamical slowdown, the origin remains to date elusive. We apply here an excess-entropy scaling strategy using molecular dynamics computer simulations and find a quasiuniversal, almost composition-independent, relation for binary mixtures, extending eight orders of magnitude in viscosi ...[more]
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