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Impact of emission reductions and meteorology changes on atmospheric mercury concentrations during the COVID-19 lockdown.

ABSTRACT: Controlling anthropogenic mercury emissions is an ongoing effort and the effect of atmospheric mercury mitigation is expected to be impacted by accelerating climate change. The lockdown measures to restrict the spread of Coronavirus Disease 2019 (COVID-19) and the following unfavorable meteorology in Beijing provided a natural experiment to examine how air mercury responds to strict control measures when the climate becomes humid and warm. Based on a high-time resolution emission inventory and generalized additive model, we found that air mercury concentration responded almost linearly to the changes in mercury emissions when excluding the impact of other factors. Existing pollution control and additional lockdown measures reduced mercury emissions by 16.7 and 12.5 kg/d during lockdown, respectively, which correspondingly reduced the concentrations of atmospheric mercury by 0.10 and 0.07 ng/m³. Emission reductions from cement clinker production contributed to the largest decrease in atmospheric mercury, implying potential mitigation effects in this sector since it is currently the number one emitter in China. However, changes in meteorology raised atmospheric mercury by 0.41 ng/m³. The increases in relative humidity (9.5%) and temperature (1.2 °C) significantly offset the effect of emission reduction by 0.17 and 0.09 ng/m³, respectively, which highlights the challenge of air mercury control in humid and warm weather and the significance of understanding mercury behavior in the atmosphere and at atmospheric interfaces, especially the impact from relative humidity.

SUBMITTER: Wu Q

PROVIDER: S-EPMC7483037 | biostudies-literature | 2021 Jan

REPOSITORIES: biostudies-literature

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Impact of emission reductions and meteorology changes on atmospheric mercury concentrations during the COVID-19 lockdown.

Wu Qingru Q Tang Yi Y Wang Long L Wang Shuxiao S Han Deming D Ouyang Daiwei D Jiang Yueqi Y Xu Peng P Xue Zhigang Z Hu Jingnan J

The Science of the total environment 20200911

Controlling anthropogenic mercury emissions is an ongoing effort and the effect of atmospheric mercury mitigation is expected to be impacted by accelerating climate change. The lockdown measures to restrict the spread of Coronavirus Disease 2019 (COVID-19) and the following unfavorable meteorology in Beijing provided a natural experiment to examine how air mercury responds to strict control measures when the climate becomes humid and warm. Based on a high-time resolution emission inventory and g ...[more]

PMID: 33182196

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Project description:Climate and air quality change due to COVID-19 lockdown (LCD) are extremely concerned subjects of several research recently. The contribution of meteorological factors and emission reduction to air pollution change over the north of Morocco has been investigated in this study using the framework generalized additive models, that have been proved to be a robust technique for the environmental data sets, focusing on main atmospheric pollutants in the region including ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2), particulate matter (PM2.5 and PM10), secondary inorganic aerosols (SIA), nom-methane volatile organic compounds and carbon monoxide (CO) from the regional air pollution dataset of the Copernicus Atmosphere Monitoring Service. Our results, indicate that secondary air pollutants (PM2.5, PM10 and O3) are more influenced by metrological factors and the other air pollutants reported by this study (NO2 and SO2). We show a negative effect for PBHL, total precipitation and NW10M on PM (PM2.5 and PM10 ), this meteorological parameters contribute to decrease in PM2.5 by 9, 2 and 9% respectively, before LCD and 8, 1 and 5% respectively during LCD. However, a positive marginal effect was found for SAT, Irradiance and RH that contribute to increase PM2.5 by 9, 12 and 18% respectively, before LCD and 17, 54 and 34% respectively during LCD. We found also that meteorological factors contribute to O3, PM2.5, PM10 and SIA average mass concentration by 22, 5, 3 and 34% before LCD and by 28, 19, 5 and 42% during LCD respectively. The increase in meteorological factors marginal effect during LCD shows the contribution of photochemical oxidation to air pollution due to increase in atmospheric oxidant (O3 and OH radical) during LCD, which can explain the response of PM to emission reduction. This study indicates that PM (PM2.5, PM10) has more controlled by SO2 due to the formation of sulfate particles especially under high oxidants level. The positive correlation between westward wind at 10 m (WW10M), Northward Wind at 10 m (NW10M) and PM indicates the implication of sea salt particles transported from Mediterranean Sea and Atlantic Ocean. The Ozone mass concentration shows a positive trend with Irradiance, Total and SAT during LCD; because temperature and irradiance enhance tropospheric ozone formation via photochemical reaction.This study shows the contribution of atmospheric oxidation capacity to air pollution change.Supplementary informationThe online version contains supplementary material available at 10.1007/s00477-022-02224-z.

Project description:The deadly transmission of the coronavirus forced all countries to implement lockdowns to restrict the transmission of this highly infectious disease. As a result of these lockdowns and restrictions, many urban centers have seen a positive impact on air quality with a significant reduction in air pollution. Therefore, in this study, the impact of COVID-19 lockdown vis-a-vis meteorological parameters on the ambient air quality of Srinagar city was examined. In this regard, we have evaluated the temporal variation of six different key air pollutants (PM10, PM2.5, SO2, NO2, O3, and NH3) along with meteorological parameters (relative humidity, rainfall, temperature, wind speed, and wind direction). The duration of the study was divided into three periods: Before Lockdown(BLD), Lockdown (LD), and Partial Lockdown(PLD). Daily average data for all the parameters was accessed from one of the real-time continuous monitoring stations of the central pollution control board (CPCB) at Rajbagh Srinagar. Some air pollutants have decreased, according to the results, while others have increased. The air quality index (AQI) decreases overall by 6.15 percent compared to before lockdown, and it never exceeds the "moderate" category. The AQI was in the following order for both lockdown and pre-lockdown periods: satisfactory > moderate > good. However, for partial lockdown, it was moderate > satisfactory > good. It was observed that the maximum decrease was seen in the concentration of NO2, NH3 with 75.11% and 69.18%. A modest decrease was observed in PM10 at 3.8%. While SO2 and O3 had an upward trend of 85.82% and 48.74%, The NO2 to SO2 ratio reveals that the emissions of NO2 have substantially decreased due to the complete restriction of transport systems. From principal component analysis for all three study periods, PM10 and PM2.5 were combined into a single component, inferring their shared behavior and source of origin. SO2 and O3 demonstrated identical behavior during the lockdown and partial lockdown periods of study. According to the findings of the study, it is beneficial for the government, environmentalists, and policymakers to impose rigorous lockdown measures, particularly during extreme air pollution events, in order to reduce the damage caused by automotive and industrial emissions.

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Dataset Information

Impact of emission reductions and meteorology changes on atmospheric mercury concentrations during the COVID-19 lockdown.

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Impact of emission reductions and meteorology changes on atmospheric mercury concentrations during the COVID-19 lockdown.

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