Giant voltage-induced modification of magnetism in micron-scale ferromagnetic metals by hydrogen charging.

ABSTRACT: Owing to electric-field screening, the modification of magnetic properties in ferromagnetic metals by applying small voltages is restricted to a few atomic layers at the surface of metals. Bulk metallic systems usually do not exhibit any magneto-electric effect. Here, we report that the magnetic properties of micron-scale ferromagnetic metals can be modulated substantially through electrochemically-controlled insertion and extraction of hydrogen atoms in metal structure. By applying voltages of only ~ 1?V, we show that the coercivity of micrometer-sized SmCo₅, as a bulk model material, can be reversibly adjusted by ~ 1?T, two orders of magnitudes larger than previously reported. Moreover, voltage-assisted magnetization reversal is demonstrated at room temperature. Our study opens up a way to control the magnetic properties in ferromagnetic metals beyond the electric-field screening length, paving its way towards practical use in magneto-electric actuation and voltage-assisted magnetic storage.

SUBMITTER: Ye X 

PROVIDER: S-EPMC7519083 | biostudies-literature | 2020 Sep

REPOSITORIES: biostudies-literature