ABSTRACT: As visible light accounts for a larger proportion of solar energy and is harmless to living organisms, it has the potential to be the energy source of micro/nanomotors, which transform visible-light energy into mechanical motion, for different applications, especially in environmental remediation. However, how to precisely control the motion of visible-light-driven micro/nanomotors (VLD-MNMs) and efficiently utilize the weak visible-light photon energy to acquire rapid motion are significant challenges. This review summarizes the most critical aspects, involving photoactive materials, propulsion mechanisms, control methods, and applications of VLD-MNMs, and discusses strategies to systematically enhance the energy-harvesting efficiency and adaptation. At first, the photoactive materials have been divided into inorganic and organic photoactive materials and comprehensively discussed. Then, different propulsion mechanisms of the current VLD-MNMs are presented to explain the improvement in the actuation force, speed, and environmental adaptability. In addition, considering the characteristics of easy control of VLD-MNMs, we summarized the direction, speed, and cluster control methods of VLD-MNMs for different application requirements. Subsequently, the potential applications of VLD-MNMs, e.g., in environmental remediation, micropumps, cargo delivery, and sensing in microscale, are presented. Finally, discussions and suggestions for future directions to enhance the energy-harvesting efficiency and adaptation of VLD-MNMs are provided.
