Thermal Hall conductivity in the cuprate Mott insulators Nd₂CuO₄ and Sr₂CuO₂Cl₂.

ABSTRACT: The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La₂CuO₄ were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar thermal Hall conductivity in two cuprate Mott insulators with significantly different crystal structures and magnetic orders - Nd₂CuO₄ and Sr₂CuO₂Cl₂ - and show that two potential mechanisms can be excluded - the scattering of phonons by rare-earth impurities and by structural domains. Our comparative study further reveals that orthorhombicity, apical oxygens, the tilting of oxygen octahedra and the canting of spins out of the CuO₂ planes are not essential to the mechanism of chirality. Our findings point to a chiral mechanism coming from a coupling of acoustic phonons to the intrinsic excitations of the CuO₂ planes.

SUBMITTER: Boulanger ME 

PROVIDER: S-EPMC7577976 | biostudies-literature | 2020 Oct

REPOSITORIES: biostudies-literature