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Dynamics of chiral solitons driven by polarized currents in monoaxial helimagnets.

ABSTRACT: Chiral solitons are one dimensional localized magnetic structures that are metastable in some ferromagnetic systems with Dzyaloshinskii-Moriya interactions and/or uniaxial magnetic anisotropy. Though topological textures in general provide a very interesting playground for new spintronics phenomena, how to properly create and control single chiral solitons is still unclear. We show here that chiral solitons in monoaxial helimagnets, characterized by a uniaxial Dzyaloshinskii-Moriya interaction, can be stabilized with external magnetic fields. Once created, the soliton moves steadily in response to a polarized electric current, provided the induced spin-transfer torque has a dissipative (nonadiabatic) component. The structure of the soliton depends on the applied current density in such a way that steady motion exists only if the applied current density is lower than a critical value, beyond which the soliton is no longer stable.

SUBMITTER: Laliena V

PROVIDER: S-EPMC7686507 | biostudies-literature | 2020 Nov

REPOSITORIES: biostudies-literature

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Dynamics of chiral solitons driven by polarized currents in monoaxial helimagnets.

Laliena Victor V Bustingorry Sebastian S Campo Javier J

Scientific reports 20201124 1

Chiral solitons are one dimensional localized magnetic structures that are metastable in some ferromagnetic systems with Dzyaloshinskii-Moriya interactions and/or uniaxial magnetic anisotropy. Though topological textures in general provide a very interesting playground for new spintronics phenomena, how to properly create and control single chiral solitons is still unclear. We show here that chiral solitons in monoaxial helimagnets, characterized by a uniaxial Dzyaloshinskii-Moriya interaction, ...[more]

PMID: 33235328

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Project description:Photon-to-matter chirality transfer offers both simplicity and universality to chiral synthesis, but its efficiency is typically low for organic compounds. Besides the fundamental importance of this process relevant for understanding the origin of homochirality on Earth, new pathways for imposing chiral bias during chemical process are essential for a variety of technologies from medicine to informatics. The strong optical activity of inorganic nanoparticles (NPs) affords photosynthetic routes to chiral superstructures using circularly polarized photons. Although plasmonic NPs are promising candidates for such synthetic routes due to the strong rotatory power of highly delocalized plasmonic states (Ma et al. Chem. Rev. 2017, 117 (12), 8041), realization of light-driven synthesis of chiral nanostructures has been more challenging for plasmonic NPs than for the semiconductor due to the short lifetime of the plasmonic states. Here we show that illumination of gold salt solutions with circularly polarized light induces the formation of NPs and their subsequent assembly into chiral nanostructures 10-15 nm in diameter. Despite their seemingly irregular shape, the resulting nanocolloids showed circular dichroism (CD) spectra with opposite polarity after exposure to photons with left and right circular polarization. The sign and spectral position of the CD peaks of illuminated dispersions matched those calculated for nanostructures with complex geometry identified from electron tomography images. Quantification of the complex shapes of NP assemblies using chirality measures revealed a direct correlation with the experimental spectra. The light-driven assembly of chiral nanostructures originates from the asymmetric displacement of NPs in dynamic assemblies by plasmonic fields followed by particle-to-particle attachment. The ability of gold NPs to "lock" the chirality of the incident photons in assembled nanostructures can be used to create a variety of chiral nanomaterials with plasmonic resonances.

Dataset Information

Dynamics of chiral solitons driven by polarized currents in monoaxial helimagnets.

Publications

Dynamics of chiral solitons driven by polarized currents in monoaxial helimagnets.

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