Dataset Information

Broadening Bandwidths of Few-Layer Absorbers by Superimposing Two High-Loss Resonators.

ABSTRACT: Efficient broadband absorption of solar radiation is desired for sea water desalination, icephobicity and other renewable energy applications. We propose an idea of superimposing two high-loss resonances to broaden bandwidths of a few-layer absorber, which is made of dielectric/ metal/dielectric/ metal layers. Both the simulation and experiment show that the structure has an averaged absorption efficiency higher than 97% at wavelengths ranging from 350 to 1200 nm. The bandwidth of the absorption larger than 90% is up to 1000 nm (410-1410 nm), which is greater than that (??750 nm) of previous MIM planar absorbers. Especially, the average absorption from 350 to 1000 nm is kept above 90% at an incidence angle as high as 65°, meanwhile still maintained above 80% even at an incident angle of 75°. The performance of angular insensitivity is much better than that of previous few-layer solar absorbers. The flexible 1D nonoble metasurface absorbers are fabricated in a single evaporation step. Under the illumination of a halogen lamp of P?=?1.2 kW/m², the flexible metasurface increases its surface temperature by 25.1 K from room temperature. Further experiments demonstrate that the heat localization rapidly melts the accumulated ice. Our illumination intensity (P?=?1.2 kW/m²) is only half of that (P?=?2.4 kW/m²) in previous solar anti-ice studies based on gold/TiO₂ particle metasurfaces, indicating that our metasurface is more advantageous topractical applications. Our results illustrate an effective pathway toward the broadband metasurface absorbers with the attractive properties of mechanical flexibility, low cost of the no-noble metals, and large-area fabrications, which have promising prospects in the applications of solar heat utilization.

SUBMITTER: Wu D

PROVIDER: S-EPMC7876209 | biostudies-literature | 2021 Feb

REPOSITORIES: biostudies-literature

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Broadening Bandwidths of Few-Layer Absorbers by Superimposing Two High-Loss Resonators.

Wu Dong D Chen Jianjun J

Nanoscale research letters 20210210 1

Efficient broadband absorption of solar radiation is desired for sea water desalination, icephobicity and other renewable energy applications. We propose an idea of superimposing two high-loss resonances to broaden bandwidths of a few-layer absorber, which is made of dielectric/ metal/dielectric/ metal layers. Both the simulation and experiment show that the structure has an averaged absorption efficiency higher than 97% at wavelengths ranging from 350 to 1200 nm. The bandwidth of the absorption ...[more]

PMID: 33566218

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Project description:The usage of flame retardants in flammable polymers has been an effective way to protect both lives and material goods from accidental fires. Phosphorus flame retardants have the potential to be follow-on flame retardants after halogenated variants, because of their low toxicity, high efficiency and compatibility. Recently, the emerging allotrope of phosphorus, two-dimensional black phosphorus, as a flame retardant has been developed. To further understand its performance in flame-retardant efficiency among phosphorus flame retardants, in this work, we built model materials to compare the flame-retardant performances of few-layer black phosphorus, red phosphorus nanoparticles, and triphenyl phosphate as flame-retardant additives in cellulose and polyacrylonitrile. Aside from the superior flame retardancy in polyacrylonitrile, few-layer black phosphorus in cellulose showed the superior flame-retardant efficiency in self-extinguishing, ~1.8 and ~4.4 times that of red phosphorus nanoparticles and triphenyl phosphate with similar lateral size and mass load (2.5~4.8 wt%), respectively. The char layer in cellulose coated with the few-layer black phosphorus after combustion was more continuous and smoother than that with red phosphorus nanoparticles, triphenyl phosphate and blank, and the amount of residues of cellulose coated with the few-layer black phosphorus in thermogravimetric analysis were 10 wt%, 14 wt% and 14 wt% more than that with red phosphorus nanoparticles, triphenyl phosphate and blank, respectively. In addition, although exothermic reactions, the combustion enthalpy changes in the few-layer black phosphorus (-127.1 kJ mol-1) are one third of that of red phosphorus nanoparticles (-381.3 kJ mol-1). Based on a joint thermodynamic, spectroscopic, and microscopic analysis, the superior flame retardancy of the few-layer black phosphorus was attributed to superior combustion reaction suppression from the two-dimensional structure and thermal nature of the few-layer black phosphorus.

Dataset Information

Broadening Bandwidths of Few-Layer Absorbers by Superimposing Two High-Loss Resonators.

Publications

Broadening Bandwidths of Few-Layer Absorbers by Superimposing Two High-Loss Resonators.

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