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Ozone chemistry and dynamics at a tropical coastal site impacted by the COVID-19 lockdown

ABSTRACT: The nationwide lockdown in India to curb the spread of Coronavirus disease 2019 (COVID-19) led to colossal reduction in anthropogenic emissions. Here, we investigated the impact of lockdown on surface ozone (O3) and nitrogen dioxide (NO2) over a tropical coastal station – Thumba, Thiruvananthapuram (8.5°N, 76.9°E). Daytime as well as night-time NO2 showed reduction by 0.8 (40%) and 2.3 (35%) ppbv, respectively during the lockdown period of 25–30 March 2020 as compared with the same period of previous 3 years. Unlike many urban locations, daytime surface O3 is found to be dramatically reduced by 15 ppbv (36%) with O3 production rate being lower by a factor of 3 during the lockdown. Interestingly, a feature of O3-hump during the onset of land breeze typically observed during 1997–1998 has reappeared with magnitude of 5–10 ppbv. A photochemical box model, capturing this feature, revealed that significant O3 sustained till onset of land breeze over the land due to weaker titration with NOx during lockdown. It is suggested that the transport of this O3 rich air with onset of land breeze led to the observed hump. Our measurements unravel a remarkable impact of the COVID-19 lockdown on the chemistry and dynamics of O3 over this tropical coastal environment.

Supplementary Information

The online version contains supplementary material available at 10.1007/s12040-021-01666-3.

SUBMITTER: Girach I

PROVIDER: S-EPMC8351570 | biostudies-literature |

REPOSITORIES: biostudies-literature

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Project description:Phase-wise variations in different aerosol (BC, AOD, PM1, PM2.5 and PM10), radiation (direct and diffused) and trace gases (NO, NO2, CO, O3, SO2, CO2 and CH4) and their associated chemistry during the COVID-19 lockdown have been investigated over a tropical rural site Gadanki (13.5° N, 79.2° E), India. Unlike most of the other reported studies on COVID-19 lockdown, this study provides variations over a unique tropical rural environment located at a scientifically strategic location in the Southern Indian peninsula. Striking differences in the time series and diurnal variability have been observed in different phases of the lockdown. The levels of most species that are primarily emitted from anthropogenic activities reduced significantly during the lockdown which also impacted the levels and diurnal variability of secondary species like O3. When compared with the same periods in 2019, short-lived trace gas species such as NO, NO2, SO2 which have direct anthropogenic emission influence have shown the reduction over 50%, whereas species like CO and O3 which have direct as well as indirect impacts of anthropogenic emissions have shown reductions up to 10%. Long-lived species (CO2 and CH4) have shown negligible difference (<1%). BC and AOD have shown reductions over 20%. Particulate Matter (1, 2.5 and 10) reductions have been in the range of 40 to 50% when compared to the pre-lockdown period. The changes in shortwave downward radiation at the surface, diffuse component due to the scattering and diffuse fraction have been +2.2%, -4.1% and -2.4%, respectively, in comparison with 2019. In contrast with the studies over urban environments, air quality category over the rural environment remained same during the lockdown despite reduction in pollutants level. All the variations observed for different species and their associated chemistry provides an excellent demonstration of rural atmospheric chemistry and its intrinsic links with the precursor concentrations and dynamics.

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Ozone chemistry and dynamics at a tropical coastal site impacted by the COVID-19 lockdown

Supplementary Information

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