Dataset Information

Investigating the Feasibility of Preparing Metal-Ceramic Multi-Layered Composites Using Only the Aerosol-Deposition Technique.

ABSTRACT: The preparation of metal-ceramic layered composites remains a challenge due to the incompatibilities of the materials at the high temperatures of the co-firing process. For densification, the ceramic thick-film materials must be subjected to high-temperature annealing (usually above 900 °C), which can increase the production costs and limit the use of substrate or co-sintering materials with a low oxidation resistance and a low melting point, such as metals. To overcome these problems, the feasibility of preparing dense, defect-free, metal-ceramic multilayers with a room-temperature-based method should be investigated. In this study, we have shown that the preparation of ceramic-metal Al2O3/Al/Al2O3/Gd multilayers using aerosol deposition (AD) is feasible and represents a simple, reliable and cost-effective approach to substrate functionalisation and protection. Scanning electron microscopy of the multilayers showed that all the layers have a dense, defect-free microstructure and good intra-layer connectivity. The top Al2O3 dielectric layer provides excellent electrical resistance (i.e., 7.7 × 1012 Ω∙m), which is required for reliable electric field applications.

SUBMITTER: Sadl M

PROVIDER: S-EPMC8400038 | biostudies-literature | 2021 Aug

REPOSITORIES: biostudies-literature

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Investigating the Feasibility of Preparing Metal-Ceramic Multi-Layered Composites Using Only the Aerosol-Deposition Technique.

Sadl Matej M Tomc Urban U Ursic Hana H

Materials (Basel, Switzerland) 20210813 16

The preparation of metal-ceramic layered composites remains a challenge due to the incompatibilities of the materials at the high temperatures of the co-firing process. For densification, the ceramic thick-film materials must be subjected to high-temperature annealing (usually above 900 °C), which can increase the production costs and limit the use of substrate or co-sintering materials with a low oxidation resistance and a low melting point, such as metals. To overcome these problems, the feasi ...[more]

PMID: 34443071

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Project description:The low deposition time efficiency and small thickness limit the expansion of polydopamine (PDA) application to fiber-reinforced high-temperature ceramic composites. In this work, the electric field-assisted polymerization (EFAP) route was developed to improve the deposition time efficiency of PDA coating and overcome the thickness limitation. Carbonized polydopamine (C-PDA) coating was used as the interphase of carbon fiber-reinforced ZrB2-based composites (Cf/ZrB2-based composite) to bond rigid fibers and brittle ceramics, where C-PDA coating was prepared by the carbonization of PDA coating. Firstly, uniform and dense PDA coatings were deposited on carbon fibers (Cf) by EFAP. The thickness of PDA coating reached the micron level (over 1800 nm) for the first time. Benefiting from the EFAP route promoting the oxidation process of dopamine (DA) and accelerating the aggregation and in-situ polymerization of DA and its derivatives on the surface of Cf, the deposition rate of PDA coating reached 5589 nm/h, which was 3 orders of magnitude higher than that of the traditional self-polymerization process. By adjusting the EFAP parameters (e.g. DA-concentration, current, and deposition time), the thickness of PDA coating could be conveniently designed from nano-scale to micro-scale. Then, PDA coating was pyrolyzed to obtain C-PDA coating. C-PDA coating was well bonded on Cf without visible cross-sticking among neighboring fibers. C-PDA coating presented a layered structure and the thickness of C-PDA coating could be designed by controlling the thickness of PDA. C-PDA coating was used as the interfacial phase of the Cf/ZrB2-based composite, which ensured that the composite possessed good load-bearing capacity and thermal stability. Moreover, extraordinary damage resistance of the composite was achieved, with work of fracture up to 9936 ± 548 J/m2 at room temperature and 19,082 ± 3458 J/m2 at 1800 °C. The current work provides a high time efficiency processing route for depositing PDA coating on carbon fibers and demonstrates the attractive potential of PDA coating in fiber-reinforced high-temperature ceramic composites.

Dataset Information

Investigating the Feasibility of Preparing Metal-Ceramic Multi-Layered Composites Using Only the Aerosol-Deposition Technique.

Publications

Investigating the Feasibility of Preparing Metal-Ceramic Multi-Layered Composites Using Only the Aerosol-Deposition Technique.

Similar Datasets

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