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Twenty-three-millisecond electron spin coherence of erbium ions in a natural-abundance crystal.


ABSTRACT: Erbium ions embedded in crystals have unique properties for quantum information processing, because of their optical transition at 1.5 μm and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most applications of erbium require, however, long electron spin coherence times, and this has so far been missing. Here, by selecting a host matrix with a low nuclear-spin density (CaWO4) and by quenching the spectral diffusion due to residual paramagnetic impurities at millikelvin temperatures, we obtain a 23-ms coherence time on the Er3+ electron spin transition. This is the longest Hahn echo electron spin coherence time measured in a material with a natural abundance of nuclear spins and on a magnetically sensitive transition. Our results establish Er3+:CaWO4 as a potential platform for quantum networks.

SUBMITTER: Le Dantec M 

PROVIDER: S-EPMC8673753 | biostudies-literature | 2021 Dec

REPOSITORIES: biostudies-literature

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Erbium ions embedded in crystals have unique properties for quantum information processing, because of their optical transition at 1.5 μm and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most applications of erbium require, however, long electron spin coherence times, and this has so far been missing. Here, by selecting a host matrix with a low nuclear-spin density (CaWO<sub>4</sub>) and by quenching the spectral diffusion due to residual paramagnetic impurit  ...[more]

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