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Magnetoelastic standing waves induced in UO2 by microsecond magnetic field pulses.


ABSTRACT: Magnetoelastic dilatometry of the piezomagnetic antiferromagnet UO2 was performed via the fiber Bragg grating method in magnetic fields up to 150 T generated by a single-turn coil setup. We show that in microsecond timescales, pulsed-magnetic fields excite mechanical resonances at temperatures ranging from 10 to 300 K, in the paramagnetic as well as within the robust antiferromagnetic state of the material. These resonances, which are barely attenuated within the 100-µs observation window, are attributed to the strong magnetoelastic coupling in UO2 combined with the high crystalline quality of the single crystal samples. They compare well with mechanical resonances obtained by a resonant ultrasound technique and superimpose on the known nonmonotonic magnetostriction background. A clear phase shift of π in the lattice oscillations is observed in the antiferromagnetic state when the magnetic field overcomes the piezomagnetic switch field H[Formula: see text] T. We present a theoretical argument that explains this unexpected behavior as a result of the reversal of the antiferromagnetic order parameter at Hc.

SUBMITTER: Schonemann R 

PROVIDER: S-EPMC8713772 | biostudies-literature | 2021 Dec

REPOSITORIES: biostudies-literature

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Magnetoelastic standing waves induced in UO<sub>2</sub> by microsecond magnetic field pulses.

Schönemann Rico R   Rodriguez George G   Rickel Dwight D   Balakirev Fedor F   McDonald Ross D RD   Evans Jordan A JA   Maiorov Boris B   Paillard Charles C   Bellaiche Laurent L   Stier Andreas V AV   Salamon Myron B MB   Gofryk Krzysztof K   Jaime Marcelo M  

Proceedings of the National Academy of Sciences of the United States of America 20211201 51


Magnetoelastic dilatometry of the piezomagnetic antiferromagnet UO<sub>2</sub> was performed via the fiber Bragg grating method in magnetic fields up to 150 T generated by a single-turn coil setup. We show that in microsecond timescales, pulsed-magnetic fields excite mechanical resonances at temperatures ranging from 10 to 300 K, in the paramagnetic as well as within the robust antiferromagnetic state of the material. These resonances, which are barely attenuated within the 100-µs observation wi  ...[more]

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