Catalytic production of low-carbon footprint sustainable natural gas.
Ontology highlight
ABSTRACT:
SUBMITTER: Si X
PROVIDER: S-EPMC8752773 | biostudies-literature |
REPOSITORIES: biostudies-literature
Similar Datasets
Project description:As natural gas demand surges in China, driven by the coal-to-gas switching policy, widespread attention is focused on its impacts on global gas supply-demand rebalance and greenhouse gas (GHG) emissions. Here, for the first time, we estimate well-to-city-gate GHG emissions of gas supplies for China, based on analyses of field-specific characteristics of 104 fields in 15 countries. Results show GHG intensities of supplies from 104 fields vary from 6.2 to 43.3 g CO2eq MJ-1. Due to the increase of GHG-intensive gas supplies from Russia, Central Asia, and domestic shale gas fields, the supply-energy-weighted average GHG intensity is projected to increase from 21.7 in 2016 to 23.3 CO2eq MJ-1 in 2030, and total well-to-city-gate emissions of gas supplies are estimated to grow by ~3 times. While securing gas supply is a top priority for the Chinese government, decreasing GHG intensity should be considered in meeting its commitment to emission reductions.
| S-EPMC7012848 | biostudies-literature
Project description:Isotopic studies have shown that many of the world's coalbed natural gas plays are secondary biogenic in origin, suggesting a potential for gas regeneration through enhanced microbial activities. The generation of biogas through biostimulation and bioaugmentation is limited to the bioavailability of coal-derived compounds and is considered carbon positive. Here we show that plant-derived carbohydrates can be used as alternative substrates for gas generation by the indigenous coal seam microorganisms. The results suggest that coalbeds can act as natural geobioreactors to produce low carbon renewable natural gas, which can be considered carbon neutral, or perhaps even carbon negative depending on the amount of carbon sequestered within the coal. In addition, coal bioavailability is no longer a limiting factor. This approach has the potential of bridging the gap between fossil fuels and renewable energy by utilizing existing coalbed natural gas infrastructure to produce low carbon renewable natural gas and reducing global warming.Coalbeds produce natural gas, which has been observed to be enhanced by in situ microbes. Here, the authors add plant-derived carbohydrates (monosaccharides) to coal seams to be converted by indigenous microbes into natural gas, thus demonstrating a potential low carbon renewable natural gas resource.
| S-EPMC5603537 | biostudies-literature
Project description:Gas fermentation offers both fossil carbon-free sustainable production of fuels and chemicals and recycling of gaseous and solid waste using gas-fermenting microbes. Bioprocess development, systems-level analysis of biocatalyst metabolism, and engineering of cell factories are advancing the widespread deployment of the commercialised technology. Acetogens are particularly attractive biocatalysts but effects of the key physiological parameter – specific growth rate (μ) – on acetogen metabolism and the gas fermentation bioprocess have not been established yet. Here, we investigate the μ-dependent bioprocess performance of the model-acetogen Clostridium autoethanogenum in CO and syngas (CO+CO2+H2) grown chemostat cultures and assess systems-level metabolic responses using gas analysis, metabolomics, transcriptomics, and metabolic modelling. We were able to obtain steady-states up to μ ~2.8 day-1 (~0.12 h-1) and show that faster growth supports both higher yields and productivities for reduced by-products ethanol and 2,3-butanediol. Transcriptomics data revealed differential expression of 1,337 genes with increasing μ and suggest that C. autoethanogenum uses transcriptional regulation to a large extent for facilitating faster growth. Metabolic modelling showed significantly increased fluxes for faster growing cells that were, however, not accompanied by gene expression changes in key catabolic pathways for CO and H2 metabolism. Cells thus seem to maintain sufficient “baseline” gene expression to rapidly respond to CO and H2 availability without delays to kick-start metabolism. Our work advances understanding of transcriptional regulation in acetogens and shows that faster growth of the biocatalyst improves the gas fermentation bioprocess.
2022-04-12 | GSE196640 | GEO
Project description:Due to the increasing environmental impact of food production, carbon footprint as an indicator can guide farmland management. This study established a method and estimated the carbon footprint of grain production in China based on life cycle analysis (LCA). The results showed that grain production has a high carbon footprint in 2013, i.e., 4052 kg ce/ha or 0.48 kg ce/kg for maize, 5455 kg ce/ha or 0.75 kg ce/kg for wheat and 11881 kg ce/ha or 1.60 kg ce/kg for rice. These footprints are higher than that of other countries, such as the United States, Canada and India. The most important factors governing carbon emissions were the application of nitrogen fertiliser (8-49%), straw burning (0-70%), energy consumption by machinery (6-40%), energy consumption for irrigation (0-44%) and CH4 emissions from rice paddies (15-73%). The most important carbon sequestration factors included returning of crop straw (41-90%), chemical nitrogen fertiliser application (10-59%) and no-till farming practices (0-10%). Different factors dominated in different crop systems in different regions. To identity site-specific key factors and take countermeasures could significantly lower carbon footprint, e.g., ban straw burning in northeast and south China, stopping continuous flooding irrigation in wheat and rice production system.
| S-EPMC5491493 | biostudies-literature
Project description:Food production in sustainable agricultural systems is one of the main challenges of modern agriculture. Vegetable intercropping may be a strategy to mitigate greenhouse gas (GHG) emissions, replacing monoculture systems. The objective is to identify the main emissions sources and to estimate GHG emissions of intercropping and monoculture production of collard greens, New Zealand spinach and chicory. Four scenarios were evaluated: ICS - intercropping collard greens and spinach; MCS - monoculture collard greens and spinach; ICC - intercropping collard greens and chicory; MCC - monoculture collard greens and chicory. The boundaries' reach from "cradle-to-gate" and the calculation of GHG emissions were performed using IPCC methodology and specific factors (Tier 2). The total GHG emitted was standardized as CO2 equivalent (CO2eq). The GHG emissions in ICS and ICC scenarios were approximately 31% lower than in MCS and MCC scenarios. Carbon footprint in ICS (0.030 kg CO2eq kg-1 vegetables year-1) and ICC (0.033 kg CO2eq kg-1 vegetables year-1) scenarios were also lower than in MCS (0.082 kg CO2eq kg-1 vegetables year-1) and MCC (0.071 kg CO2eq kg-1 vegetables year-1) scenarios. Fertilizers, fuel (diesel) and irrigation were the main contributing sources for total GHG emitted and carbon footprint in all evaluated scenarios. The results suggest that intercropping systems may reduce GHG emissions associated with the production of vegetables evaluated as compared with monoculture.
| S-EPMC9667872 | biostudies-literature
Project description:Eighty percent of US oil and natural gas (O&G) production sites are low production well sites, with average site-level production ≤15 barrels of oil equivalent per day and producing only 6% of the nation's O&G output in 2019. Here, we integrate national site-level O&G production data and previously reported site-level CH4 measurement data (n = 240) and find that low production well sites are a disproportionately large source of US O&G well site CH4 emissions, emitting more than 4 (95% confidence interval: 3-6) teragrams, 50% more than the total CH4 emissions from the Permian Basin, one of the world's largest O&G producing regions. We estimate low production well sites represent roughly half (37-75%) of all O&G well site CH4 emissions, and a production-normalized CH4 loss rate of more than 10%-a factor of 6-12 times higher than the mean CH4 loss rate of 1.5% for all O&G well sites in the US. Our work suggests that achieving significant reductions in O&G CH4 emissions will require mitigation of emissions from low production well sites.
| S-EPMC9019036 | biostudies-literature
Project description:Wheat is one of the world's most favoured food sources, reaching millions of people on a daily basis. However, its production has climatic consequences. Fuel, inorganic fertilizers and pesticides used in wheat production emit greenhouse gases that can contribute negatively to climate change. It is unknown whether adopting alternative farming practices will increase crop yield while reducing carbon emissions. Here we quantify the carbon footprint of alternative wheat production systems suited to semiarid environments. We find that integrating improved farming practices (that is, fertilizing crops based on soil tests, reducing summerfallow frequencies and rotating cereals with grain legumes) lowers wheat carbon footprint effectively, averaging -256 kg CO2 eq ha(-1) per year. For each kg of wheat grain produced, a net 0.027-0.377 kg CO2 eq is sequestered into the soil. With the suite of improved farming practices, wheat takes up more CO2 from the atmosphere than is actually emitted during its production.
| S-EPMC4243251 | biostudies-literature
Project description:As a major agricultural country, the comprehensive accounting of the dynamics and composition of the carbon footprint of major crops in China will provide a decision-making basis for environmental management and agricultural green development in the whole process of the major crop production system in China. To investigate the spatiotemporal dynamics of the carbon footprint for major crops in China, a life cycle-based carbon footprint approach was used to evaluate the carbon footprint per unit area (CFA) and per unit yield (CFY) of eight crops for the period of 1990 to 2019. Our results showed that the CFA for all major crops showed an increasing trend with time before 2016 but slowly decreased afterward, while the CFY decreased by 16-43% over the past 30 years due to the increase in crop yield. The three main grain crops, rice (4871 ± 418 kg CO2-eq · ha-1), wheat (2766 ± 552 kg CO2-eq · ha-1), and maize (2439 ± 530 kg CO2-eq · ha-1), showed the highest carbon footprint and contribution to the total greenhouse gas (GHG) emissions, mainly due to their larger cultivated areas and higher fertilizer application rates. CH4 emission was the major component of the carbon footprint for rice production, accounting for 66% and 48% of the CFA and CFY, respectively, while fertilizer production and usage were the largest components of carbon footprint for dryland crops, making up to 26-49% of the CFA and 26-50% of the CFY for different crops. The present study also highlighted the spatial and temporal patterns of the carbon footprint for major crops in China, which could serve as references for the development of best management practices for different crop production in China, to mitigate agricultural GHG emission and to pursue low-carbon agriculture.
| S-EPMC9658409 | biostudies-literature
Project description:Considering the importance of sustainable nutrition, it is important that hospitals' meal menus are planned to ensure the lowest possible environmental footprint. In this study, we aimed to evaluate the environmental effects of hospital menus and the changes that may occur when these menus are planned according to the Turkey Dietary Guidelines and Mediterranean diet recommendations. In this context, first, the yearly environmental footprints of the standard meal menus of the state university hospitals in Turkey (n = 42), including water footprint (WF) and greenhouse gas emission (GHGE) values, were determined. Second, changes in the environmental footprint as a result of arranging the standard meal menus of state university hospitals according to the Turkey Dietary Guidelines and Mediterranean nutritional models were evaluated. It was determined that the average WF and GHGE values of hospital menus were 137,280 ± 18537.2 L/month and 140.0 ± 18.4 kg CO2-eq/month, respectively. Adjusting state university hospitals' standard meal menus according to Turkey Dietary Guidelines and Mediterranean nutritional models reduced WF by 24.8% to 103206.7 L/month and 37.8% to 85420.5 L/month, and GHGEs by 31.7% to 95.5 kg CO2-eq/month and 49% to 71.3 kg CO2-eq/month, respectively. In addition, it was determined that hospital meal menus planned according to the Turkey Dietary Guidelines and the Mediterranean nutritional model contained lower saturated fat and cholesterol and higher dietary fiber. In conclusion, planning hospital menus according to the Turkey Dietary Guidelines and Mediterranean nutritional recommendations can reduce the environmental footprint of hospital food services.
| S-EPMC11317658 | biostudies-literature
Project description:Natural gas combined-cycle (NGCC) turbines with carbon capture and storage (CCS) could be an important source of low-carbon electricity in the future. Factors affecting the market competitiveness of NGCC-CCS are examined by conducting a sensitivity analysis using the MARKet ALlocation energy system optimization model. The results indicate that widespread deployment of NGCC-CCS is better suited for a 30% energy system greenhouse gas (GHG) reduction trajectory than for a more stringent 50% reduction trajectory. Methane leakage rate, efficiency penalty, carbon dioxide (CO2) capture rate, and natural gas price are found to be the strongest factors influencing optimal NGCC-CCS deployment, in that order. NGCC plays an important role in meeting mid-term GHG targets across all model runs. A large portion of NGCC capacity is later retrofit with CCS, indicating that NGCC can be both a bridge to a low-carbon future and an integral part of that future. Thus, retrofitability and siting near CO2storage should be considerations as new NGCC capacity is built. Regional results indicate that NGCC-CCS deployment would be greatest in the West South Central region, followed by the East North Central region. In a business-as-usual scenario, both regions have considerable electricity production from fossil fuels. Conventional coal and gas capacity are displaced under a GHG reduction target, opening the door for NGCC-CCS in these regions. NGCC-CCS market penetration is projected to have a mixed impact on air pollutant emissions and energy-related water consumption. Whether impacts are positive or negative depends on the technologies displaced by NGCC-CCS.
| S-EPMC7252577 | biostudies-literature