Life Cycle Environmental Impacts of Wastewater-Derived Phosphorus Products: An Agricultural End-User Perspective.
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ABSTRACT:
SUBMITTER: Lam KL
PROVIDER: S-EPMC9301919 | biostudies-literature |
REPOSITORIES: biostudies-literature
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Project description:Environmental data on organic products are needed to assess their environmental performance. The purpose of the ACV Bio project reported here was to generate environmental data as life cycle assessment (LCA) data for a sample of French organic production systems including cropping systems (annual crops, intercrops, forages), grassland, wine grapes, cow milk, calves, beef cattle, sheep, pigs, broilers and eggs. LCA was used to estimate environmental impacts of products from these systems. Recommended uses are to characterize part of the diversity of French organic farming systems and some of their environmental impacts, identify areas for improvement, perform eco-design and sensitivity analysis, and/or make system choices in a given context. However, these data do not represent average French organic products and should not be used as such. The MEANS-InOut web application was used to generate life cycle inventories (LCI). Impact assessment was performed using SimaPro v9 software. The Environmental Footprint 2.0 characterisation method was used to generate LCA data. These data were supplemented with three LCA indicators: cumulative energy demand, land competition (CML-IA non-baseline) and biodiversity loss. Three non-LCA indicators were also calculated for certain systems: diversity of crop families (for cropping systems), agro-ecological infrastructure (for sheep) and pesticide treatment frequency index (for grapes). In total, 173 products were modelled. LCA and non-LCA data are available in the Microsoft® Excel file at Data INRAE (https://doi.org/10.15454/TTR25S). LCI data are available in the AGRIBALYSE database and can be accessed using SimaPro and openLCA software. Farmer-practice data are available on demand.
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Project description:Phosphorus (P) fertilizer has contributed to the eutrophication of freshwater ecosystems. Watershed-based conservation programs aiming to reduce external P loading to surface waters have not resulted in significant water-quality improvements. One factor that can help explain the lack of water-quality response is remobilization of accumulated legacy (historical) P within the terrestrial-aquatic continuum, which can obscure the beneficial impacts of current conservation efforts. We examined how contemporary river P trends (between 1992 and 2012) responded to estimated changes in contemporary agricultural P balances [(fertilizer + manure inputs)-crop uptake and harvest removal] for 143 watersheds in the conterminous United States, while also developing a proxy estimate of legacy P contribution, which refers to anthropogenic P inputs before 1992. We concluded that legacy sources contributed to river export in 49 watersheds because mean contemporary river P export exceeded mean contemporary agricultural P balances. For the other 94 watersheds, agricultural P balances exceeded river P export, and our proxy estimate of legacy P was inconclusive. If legacy contributions occurred in these locations, they were likely small and dwarfed by contemporary P sources. Our continental-scale P mass balance results indicated that improved incentives and strategies are needed to promote the adoption of nutrient-conserving practices and reduce widespread contemporary P surpluses. However, a P surplus reduction is only 1 component of an effective nutrient plan as we found agricultural balances decreased in 91 watersheds with no consistent water-quality improvements, and balances increased in 52 watersheds with no consistent water-quality degradation.
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Project description:Understanding and communicating the environmental impacts of food products is key to enabling transitions to environmentally sustainable food systems [El Bilali and Allahyari, Inf. Process. Agric. 5, 456-464 (2018)]. While previous analyses compared the impacts of food commodities such as fruits, wheat, and beef [Poore and Nemecek, Science 360, 987-992 (2018)], most food products contain numerous ingredients. However, because the amount of each ingredient in a product is often known only by the manufacturer, it has been difficult to assess their environmental impacts. Here, we develop an approach to overcome this limitation. It uses prior knowledge from ingredient lists to infer the composition of each ingredient, and then pairs this with environmental databases [Poore and Nemecek Science 360, 987-992 (2018); Gephart et al., Nature 597, 360-365 (2021)] to derive estimates of a food product's environmental impact across four indicators: greenhouse gas emissions, land use, water stress, and eutrophication potential. Using the approach on 57,000 products in the United Kingdom and Ireland shows food types have low (e.g., sugary beverages, fruits, breads), to intermediate (e.g., many desserts, pastries), to high environmental impacts (e.g., meat, fish, cheese). Incorporating NutriScore reveals more nutritious products are often more environmentally sustainable but there are exceptions to this trend, and foods consumers may view as substitutable can have markedly different impacts. Sensitivity analyses indicate the approach is robust to uncertainty in ingredient composition and in most cases sourcing. This approach provides a step toward enabling consumers, retailers, and policy makers to make informed decisions on the environmental impacts of food products.
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Project description:PurposeMany people do not participate in mail-out bowel cancer screening programs due to difficulties using the screening kit. The current study investigated the ways the screening kit could be modified to improve usability.Methods1,109 people evaluated 15 different screening kit modifications. Participants reported on how these kit modifications would affect their screening barriers, their future screening intentions, and how much they would recommend that the modification is made to the current screening kit used the program. All responses were given via an online survey conducted between April and December of 2021.ResultsSeventeen percent of previous NBCSP non-participators indicated that a one-sample test would increase their intention to participate. Recommendation ratings demonstrated higher levels of support for modifications that included providing a barcode naming label (M = 9.06, 95% CI [8.81, 9.31]), having a larger diameter opening of the collection tube (M = 8.42, 95% CI [8.10, 8.74]), and highlighting the expiry date on the kit packaging (M = 8.59, 95% CI [8.29, 8.89]). There were lower levels of support for modifications that reduced the size of the packaging the kit is sent in (M = 6.47, 95% CI [6.09, 6.85]), removed branding from kit packaging (M = 5.98, 95% CI [5.57, 6.39]), and removed the information booklet that comes with the screening kit (M = 5.25, 95% CI [4.78, 5.72]).ConclusionThese findings highlight multiple ways in which bowel cancer screening kits can be changed to increase usability for invitees of national bowel cancer screening programs. Findings have implications for all screening programs that use immunochemical-based bowel cancer screening kits.
| S-EPMC10202976 | biostudies-literature
Project description:BackgroundMicroalgae are touted as an attractive alternative to traditional forms of biomass for biofuel production, due to high productivity, ability to be cultivated on marginal lands, and potential to utilize carbon dioxide (CO2) from industrial flue gas. This work examines the fossil energy return on investment (EROIfossil), greenhouse gas (GHG) emissions, and direct Water Demands (WD) of producing dried algal biomass through the cultivation of microalgae in Open Raceway Ponds (ORP) for 21 geographic locations in the contiguous United States (U.S.). For each location, comprehensive life cycle assessment (LCA) is performed for multiple microalgal biomass production pathways, consisting of a combination of cultivation and harvesting options.ResultsResults indicate that the EROIfossil for microalgae biomass vary from 0.38 to 1.08 with life cycle GHG emissions of -46.2 to 48.9 (g CO2 eq/MJ-biomass) and direct WDs of 20.8 to 38.8 (Liters/MJ-biomass) over the range of scenarios analyzed. Further anaylsis reveals that the EROIfossil for production pathways is relatively location invariant, and that algae's life cycle energy balance and GHG impacts are highly dependent on cultivation and harvesting parameters. Contrarily, algae's direct water demands were found to be highly sensitive to geographic location, and thus may be a constraining factor in sustainable algal-derived biofuel production. Additionally, scenarios with promising EROIfossil and GHG emissions profiles are plagued with high technological uncertainty.ConclusionsGiven the high variability in microalgae's energy and environmental performance, careful evaluation of the algae-to-fuel supply chain is necessary to ensure the long-term sustainability of emerging algal biofuel systems. Alternative production scenarios and technologies may have the potential to reduce the critical demands of biomass production, and should be considered to make algae a viable and more efficient biofuel alternative.
| S-EPMC3693881 | biostudies-literature
Project description:The current debate on the sustainability of bio-based products questions the environmental benefits of replacing fossil- by bio-resources. Here, we analyze the environmental trade-offs of 98 emerging bio-based materials compared to their fossil counterparts, reported in 130 studies. Although greenhouse gas life cycle emissions for emerging bio-based products are on average 45% lower (-52 to -37%; 95% confidence interval), we found a large variation between individual bio-based products with none of them reaching net-zero emissions. Grouped in product categories, reductions in greenhouse gas emissions ranged from 19% (-52 to 35%) for bioadhesives to 73% (-84 to -54%) for biorefinery products. In terms of other environmental impacts, we found evidence for an increase in eutrophication (369%; 163 to 737%), indicating that environmental trade-offs should not be overlooked. Our findings imply that the environmental sustainability of bio-based products should be evaluated on an individual product basis and that more radical product developments are required to reach climate-neutral targets.
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Project description:Despite concerns about the potential risk associated with the environmental occurrence of pharmaceuticals and personal care products (PPCPs), few studies address the emissions of hospitals to aquatic compartments. We examined within a 3-month sampling period the occurrence and environmental risk of PPCPs in seven Tunisian hospital wastewaters. From personal care products, UV filters, main metabolites, and benzotriazoles were quantified, with benzophenone 3 (oxybenzone, BP3) and benzotriazole (BZT) the most frequently found (71%) at median concentrations in the range 2.43 ± 0.87 ngL-1-64.05 ± 6.82 ngL-1 for BP3 and 51.67 ± 1.67 ngL-1-254 ± 9.9 ngL-1 for BZT. High concentrations were also found for 4-hydroxybenzophenone (4HB) (221 ± 6.22 ngL-1), one of the main metabolites of BP3. The antibiotics ofloxacin and trimethoprim, the anti-inflammatory acetaminophen, the antiepileptic carbamazepine, and the stimulant caffeine were present in all the wastewaters. The highest median concentration corresponded to acetaminophen, with 1240 ± 94 mgL-1 in Tunis Hospital, followed by ofloxacin with 78850 ± 39 μgL-1 in Sousse Hospital. For ecotoxicity assessment, acute toxicity was observed for Daphnia magna and Vibrio fischeri. The toxicity data were used in a hazard quotient (HQ) approach to evaluate the risk posed by the target PPCPs to aquatic organisms. The calculated HQs revealed that marbofloxacin (234 for V. fischeri), enrofloxacin (121 for D. magna), and BZT (82.2 for D. magna and 83.7 for V. fischeri) posed the highest risk, concluding that potential risk exists toward aquatic microorganisms. This study constitutes the first monitoring of UV filters in Tunisian hospital effluents and provides occurrence and toxicity data of PPCPs for reference in further surveys in the country.
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Project description:The recovery of phosphorus (P) from high-strength acidic waste streams with high salinity and organic loads is challenging. Here, we addressed this challenge with a recently developed electrochemical approach and compared it with the chemical precipitation method via NaOH dosing. The electrochemical process recovers nearly 90% of P (∼820 mg/L) from cheese wastewater in 48 h at 300 mA with an energy consumption of 64.7 kWh/kg of P. With chemical precipitation, >86% of P was removed by NaOH dosing with a normalized cost of 1.34-1.80 euros/kg of P. The increase in wastewater pH caused by NaOH dosing triggered the formation of calcium phosphate sludge instead of condensed solids. However, by electrochemical precipitation, the formed calcium phosphate is attached to the electrode, allowing the subsequent collection of solids from the electrode after treatment. The collected solids are characterized as amorphous calcium phosphate (ACP) at 200 mA or a precipitation pH of ≥9. Otherwise, they are a mixture of ACP and hydroxyapatite. The products have sufficient P content (≤14%), of which up to 85% was released within 30 min in 2% citric acid and a tiny amount of heavy metals compared to phosphate rocks. This study paves the way for applying electrochemical removal and recovery of phosphorus from acidic P-rich wastewater and offers a sustainable substitute for mined phosphorus.
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Project description:Phosphate rock (PR) has been designated as a Critical Raw Material in the European Union (EU). This has led to increased emphasis on alternative P recovery (APR) from secondary streams like wastewater sludge (WWS). However, WWS end-use is a contentious topic, and EU member states prefer different end-use pathways (land application/incineration/valorisation in cement kilns). Previous Life Cycle Assessments (LCA) on APRs from WWS reached contrasting conclusions; while most considered WWS as waste and highlighted a net benefit relative to PR mining and beneficiation, others viewed WWS as a resource and highlighted a net burden of the treatment. We used a combined functional unit (that views WWS from a waste as well as a resource perspective) and applied it on a Flemish wastewater treatment plant (WWTP) with struvite recovery as APR technology. Firstly, a retrospective comparison was performed to measure the WWTP performance before and after struvite recovery and the analysis was complemented by uncertainty and global sensitivity analyses. The results showed struvite recovery provides marginal environmental benefits due to improved WWS dewatering and reduced polymer use. Secondly, a prospective LCA approach was performed to reflect policy changes regarding WWS end-use options in Flanders. Results indicated complete mono-incineration of WWS, ash processing to recover P and the subsequent land application appears to be less sustainable in terms of climate change, human toxicity, and terrestrial acidification relative to the status quo, i.e., co-incineration with municipal solid waste and valorisation at cement kilns. Impacts on fossil depletion, however, favour mono-incineration over the status quo.
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Project description:This study estimates the life cycle water consumption and wastewater generation impacts of a Marcellus shale gas well from its construction to end of life. Direct water consumption at the well site was assessed by analysis of data from approximately 500 individual well completion reports collected in 2010 by the Pennsylvania Department of Conservation and Natural Resources. Indirect water consumption for supply chain production at each life cycle stage of the well was estimated using the economic input-output life cycle assessment (EIO-LCA) method. Life cycle direct and indirect water quality pollution impacts were assessed and compared using the tool for the reduction and assessment of chemical and other environmental impacts (TRACI). Wastewater treatment cost was proposed as an additional indicator for water quality pollution impacts from shale gas well wastewater. Four water management scenarios for Marcellus shale well wastewater were assessed: current conditions in Pennsylvania; complete discharge; direct reuse and desalination; and complete desalination. The results show that under the current conditions, an average Marcellus shale gas well consumes 20,000 m(3) (with a range from 6700 to 33,000 m(3)) of freshwater per well over its life cycle excluding final gas utilization, with 65% direct water consumption at the well site and 35% indirect water consumption across the supply chain production. If all flowback and produced water is released into the environment without treatment, direct wastewater from a Marcellus shale gas well is estimated to have 300-3000 kg N-eq eutrophication potential, 900-23,000 kg 2,4D-eq freshwater ecotoxicity potential, 0-370 kg benzene-eq carcinogenic potential, and 2800-71,000 MT toluene-eq noncarcinogenic potential. The potential toxicity of the chemicals in the wastewater from the well site exceeds those associated with supply chain production, except for carcinogenic effects. If all the Marcellus shale well wastewater is treated to surface discharge standards by desalination, $59,000-270,000 per well would be required. The life cycle study results indicate that when gas end use is not considered hydraulic fracturing is the largest contributor to the life cycle water impacts of a Marcellus shale gas well.
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